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Chemistry - A European Journal

Tumor Targeting with an iso DGR–Drug Conjugate

Published: 26 May 2017

Author(s): Simone Zanella, Simona Angerani, Arianna Pina, Paula López Rivas, Clelia Giannini, Silvia Panzeri, Daniela Arosio, Michele Caruso, Fabio Gasparri, Ivan Fraietta, Clara Albanese, Aurelio Marsiglio, Luca Pignataro, Laura Belvisi, Umberto Piarulli, Cesare Gennari

Abstract Herein we report the first example of an isoDGR–drug conjugate (2), designed to release paclitaxel selectively within cancer cells expressing integrin αVβ3. Conjugate 2 was synthesized by connecting the isoDGR peptidomimetic 5 with paclitaxel via the lysosomally cleavable Val–Ala dipeptide linker. Conjugate 2 displayed a low nanomolar affinity for the purified integrin αVβ3 receptor (IC50=11.0 nm). The tumor targeting ability of conjugate 2 was assessed in...

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Sequence‐Specific Covalent Capture Coupled with High‐Contrast Nanopore Detection of a Disease‐Derived Nucleic Acid Sequence

Published: 26 May 2017

Author(s): Maryam Imani Nejad, Ruicheng Shi, Xinyue Zhang, Li‐Qun Gu, Kent S. Gates

Abstract Hybridization‐based methods for the detection of nucleic acid sequences are important in research and medicine. Short probes provide sequence specificity, but do not always provide a durable signal. Sequence‐specific covalent crosslink formation can anchor probes to target DNA and might also provide an additional layer of target selectivity. Here, we developed a new crosslinking reaction for the covalent capture of specific...

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Chemistry - A European Journal

Metal‐Free Arene and Heteroarene Borylation Catalyzed by Strongly Electrophilic Bis‐boranes

Published: 26 May 2017

Author(s): Yun‐Lin Liu, Gerald Kehr, Constantin G. Daniliuc, Gerhard Erker

Abstract The geminal chelate bis‐borylalkanes 4 and 5 featuring strongly electrophilic B(C6F5)2 and B(C6F5) groups, respectively, serve as efficient catalysts for the borylation of arenes and heteroarenes. The borylation reactions proceed under mild conditions with liberation of dihydrogen.

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β‐Octabromo‐ and β‐Octakis(trifluoromethyl)isocorroles: New Sterically Constrained Macrocyclic Ligands

Published: 26 May 2017

Author(s): Kolle E. Thomas, Christine M. Beavers, Kevin J. Gagnon, Abhik Ghosh

Abstract Presented herein is a study of the acid‐induced demetalation of two sterically hindered copper corroles, Cu β‐octabromo‐meso‐triphenylcorrole (Cu[Br8TPC]) and β‐octakis(trifluoromethyl)‐meso‐tris(p‐methoxyphenyl)corrole (Cu[(CF3)8TpOMePC]). Unlike reductive demetalation, which affords the free‐base β‐octabromocorrole, demetalation of Cu[Br8TPC] under non‐ reductive conditions (CHCl3/H2SO4) resulted in moderate yields of free‐base 5‐ and 10‐hydroxy...


Catalytic Hydrogenation of Arenes in Water Over In Situ Generated Ruthenium Nanoparticles Immobilized on Carbon

Published: 26 May 2017

Author(s): Ambikesh Dhar Dwivedi, Rohit Kumar Rai, Kavita Gupta, Sanjay Kumar Singh

Abstract We describe a tandem process to generate active Ru nanoparticles (≈7 nm) immobilised in situ on carbon from an organometallic precursor and formic acid to afford the hydrogenation of a wide range of arenes and heteroarenes in yields up to 72 % with high conversions and selectivities for the desired products. The hydrogenation of several substrates analogous to lignin‐derived fragments to the corresponding alicyclic products...

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Chemistry - A European Journal

d ‐Cysteine Ligands Control Metal Geometries within De Novo Designed Three‐Stranded Coiled Coils

Published: 26 May 2017

Author(s): Leela Ruckthong, Anna F. A. Peacock, Cherilyn E. Pascoe, Lars Hemmingsen, Jeanne A. Stuckey, Vincent L. Pecoraro

Abstract Although metal ion binding to naturally occurring l‐amino acid proteins is well documented, understanding the impact of the opposite chirality (d‐)amino acids on the structure and stereochemistry of metals is in its infancy. We examine the effect of a d‐configuration cysteine within a designed l‐amino acid three‐stranded coiled coil in order to enforce a precise coordination number on a metal center. The d chirality does not alter the native fold, but the...

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Chemistry - A European Journal

Liquid/Liquid Interfacial Synthesis of a Click Nanosheet

Published: 26 May 2017

Author(s): Amalia Rapakousiou, Ryota Sakamoto, Ryo Shiotsuki, Ryota Matsuoka, Ukyo Nakajima, Tigmansu Pal, Rintaro Shimada, Amran Hossain, Hiroyasu Masunaga, Satoshi Horike, Yasutaka Kitagawa, Sono Sasaki, Kenichi Kato, Takeaki Ozawa, Didier Astruc, Hiroshi Nishihara

Abstract A liquid/liquid interfacial synthesis is employed, for the first time, to synthesize a covalent two‐dimensional polymer nanosheet. Copper‐catalyzed azide–alkyne cycloaddition (CuAAC) between a three‐way terminal alkyne and azide at a water/dichloromethane interface generates a 1,2,3‐triazole‐linked nanosheet. The resultant nanosheet, with a flat and smooth texture, has a maximum domain size of 20 μm and minimum thickness of...

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Chemistry - A European Journal

Mechanistic Aspects in the Formation, Growth and Surface Functionalization of Metal Oxide Nanoparticles in Organic Solvents

Published: 26 May 2017

Author(s): Rupali Deshmukh, Markus Niederberger

Abstract The synthesis of metal oxide nanoparticles in organic solvents, so‐called nonaqueous (or nonhydrolytic) processes represent powerful alternatives to aqueous approaches and have become an independent research field. 10 Years ago, when we published our first review on organic reaction pathways in nonaqueous sol–gel approaches, the number of examples was relatively limited. Nowadays, it is almost impossible to provide an exhaustive...

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Chemistry - A European Journal

Heterotetracenes: Flexible Synthesis and in Silico Assessment of the Hole‐Transport Properties

Published: 26 May 2017

Author(s): Yifan Li, Ganna Gryn'ova, Felipe Saenz, Xavier Jeanbourquin, Kevin Sivula, Clémence Corminboeuf, Jérôme Waser

Abstract Thienoacenes and furoacenes are among the most frequent molecular units found in organic materials. The efficient synthesis of morphologically different heteroacenes and the rapid determination of their solid‐state and electronic properties are still challenging tasks, which slow down progress in the development of new materials. Here, we report a flexible and efficient synthesis of unprecedented heterotetracenes based on a...

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Chemistry - A European Journal

Photoelectrochemical Catalysis toward Selective Anaerobic Oxidation of Alcohols

Published: 24 May 2017

Author(s): Ruikang Zhang, Mingfei Shao, Zhenhua Li, Fanyu Ning, Min Wei, David G. Evans, Xue Duan

Abstract Selective oxidation of alcohols to aldehydes plays an important role in perfumery, pharmaceuticals, and agrochemicals industry. Different from traditional catalysis or photocatalytic process, here we report an effective photoelectrochemical (PEC) approach for selective anaerobic oxidation of alcohols accompanied with H2 production by means of solar energy. By using TiO2 nanowires modified with graphitic carbon layer as photoanode,...

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Most-accessed articles from each ChemPubSoc Europe, ACES, and GDCh journal

April 2017


Xin Mu, Yu Shibata, Yusuke Makida, Gregory C. Fu
Control of Vicinal Stereocenters through Nickel‐Catalyzed Alkyl–Alkyl Cross‐Coupling [Communication]
Angew. Chem. Int. Ed. 2017, vol. 56, p. 5821

Dario Neri
Twenty‐five Years of DNA‐Encoded Chemical Libraries [Editorial]
ChemBioChem 2017, vol. 18, p. 827

Isabela C. Man, Hai‐Yan Su, Federico Calle‐Vallejo, Heine A. Hansen, José I. Martínez, Nilay G. Inoglu, John Kitchin, Thomas F. Jaramillo, Jens K. Nørskov, Jan Rossmeisl
Universality in Oxygen Evolution Electrocatalysis on Oxide Surfaces [Full Paper]
ChemCatChem 2011, vol. 3, p. 1159

Warum brennt Alkohol eigentlich in Wunden? [Treffpunkt Forschung]
Chem. Unserer Zeit 2017, vol. 51, p. 83

Thammadihalli Nanjundaiah Ravishankar, Thippeswamy Ramakrishnappa, Ganganagappa Nagaraju, Hanumanaika Rajanaika
Synthesis and Characterization of CeO2 Nanoparticles via Solution Combustion Method for Photocatalytic and Antibacterial Activity Studies [Full Paper]
ChemistryOpen 2015, vol. 4, p. 146

Hanshen Xin, Xike Gao
Application of Azulene in Constructing Organic Optoelectronic Materials: New Tricks for an Old Dog [Minireview]
ChemPlusChem 2017, 10.1002/cplu.201700039

Yang Song, Rui Peng, Dale K. Hensley, Peter V. Bonnesen, Liangbo Liang, Zili Wu, Harry M. Meyer, Miaofang Chi, Cheng Ma, Bobby G. Sumpter, Adam J. Rondinone
High‐Selectivity Electrochemical Conversion of CO2 to Ethanol using a Copper Nanoparticle/N‐Doped Graphene Electrode [Full Paper]
ChemistrySelect 2016, 10.1002/slct.201601169

Hubert Rauscher, Kirsten Rasmussen, Birgit Sokull‐Klüttgen
Regulatory Aspects of Nanomaterials in the EU [Research Article]
Chem. Ing. Tech. 2017, vol. 89, p. 224

Abas Mohsenzadeh, Akram Zamani, Mohammad J. Taherzadeh
Bioethylene Production from Ethanol: A Review and Techno‐economical Evaluation [Review]
ChemBioEng Rev. 2017, vol. 4, p. 75

Joanne Tory, Briony Setterfield‐Price, Robert A. W. Dryfe, František Hartl
[M(CO)4(2,2′‐bipyridine)] (M=Cr, Mo, W) Complexes as Efficient Catalysts for Electrochemical Reduction of CO2 at a Gold Electrode [Communication]
ChemElectroChem 2015, vol. 2, p. 213

Elke Debroye, Haifeng Yuan, Eva Bladt, Wouter Baekelant, Mark Van der Auweraer, Johan Hofkens, Sara Bals, Maarten B. J. Roeffaers
Facile Morphology‐Controlled Synthesis of Organolead Iodide Perovskite Nanocrystals Using Binary Capping Agents [Communication]
ChemNanoMat 2017, 10.1002/cnma.201700006

Hirotatsu Umihara, Satoshi Yokoshima, Masayuki Inoue, Tohru Fukuyama
Total Synthesis of (−)‐Morphine [Communication]
Chem. Eur. J. 2017, 10.1002/chem.201701438

Sandip G. Agalave, Suleman R. Maujan, Vandana S. Pore
Click Chemistry: 1,2,3‐Triazoles as Pharmacophores [Focus Review]
Chem. Asian J. 2011, vol. 6, p. 2696

Edward J. Emmett, Michael C. Willis
The Development and Application of Sulfur Dioxide Surrogates in Synthetic Organic Chemistry [Focus Review]
Asian J. Org. Chem. 2015, vol. 4, p. 602

Yves P. Auberson, Cara Brocklehurst, Markus Furegati, Thomas C. Fessard, Guido Koch, Andrea Decker, Luigi La Vecchia, Emmanuelle Briard
Improving Nonspecific Binding and Solubility: Bicycloalkyl Groups and Cubanes as para‐Phenyl Bioisosteres [Full Paper]
ChemMedChem 2017, vol. 12, p. 590

Jamie Gibson, Andrew Monkman, Thomas Penfold
The Importance of Vibronic Coupling for Efficient Reverse Intersystem Crossing in TADF molecules [Communication]
ChemPhysChem 2016, 10.1002/cphc.201600662

Jia‐Rong Chen, Dong‐Mei Yan, Qiang Wei, Wen‐Jing Xiao
Photocascade Catalysis: A New Strategy for Cascade Reactions [Concept]
ChemPhotoChem 2017, 10.1002/cptc.201700008

Arjan W. Kleij, Michael North, Atsushi Urakawa
CO2 Catalysis [Editorial]
ChemSusChem 2017, 10.1002/cssc.201700218

Ross J. Marshall, Ross S. Forgan
Postsynthetic Modification of Zirconium Metal‐Organic Frameworks [Microreview]
Eur. J. Inorg. Chem. 2016, 10.1002/ejic.201600394

Burkhard König
Photocatalysis in Organic Synthesis – Past, Present, and Future [Essay]
Eur. J. Org. Chem. 2017, p. 1979

T. Henle
Historisches zur Lebensmittelchemie an der TU Dresden [Artikel]
Lebensmittelchemie 2017, vol. 71, p. 20

Frauke Zbikowski
Vom emissionsfreien Kamin und musikalischen Molekül [Bildung & Gesellschaft]
Nachr. Chem. 2017, vol. 65, p. 478

Katrin Sommer, Christina Toschka, Laura Schröder, Thomas Philipp Schröder, Henning Steff, Roland A. Fischer
Modellexperimente im Chemieunterricht. [Artikel]
CHEMKON 2017, vol. 24, p. 13

Sarah Millar
Tips and Tricks for the Lab: Column Choices
ChemViews Magazine 2012.

Most Cited articles from ChemPubSoc Europe, ACES, and GDCh journals



Shoujun Zhu, Qingnan Meng, Lei Wang, Junhu Zhang, Yubin Song, Han Jin, Kai Zhang, Hongchen Sun, Haiyu Wang, Bai Yang
Highly Photoluminescent Carbon Dots for Multicolor Patterning, Sensors, and Bioimaging
Angew. Chem. Int. Ed. 2013, vol. 52, pp. 3953–3957

Naohiko Yoshikai, Ye Wei
Synthesis of Pyrroles, Indoles, and Carbazoles through Transition-Metal-Catalyzed C–H Functionalization [Review]
Asian J. Org. Chem. 2013, vol. 2, pp. 466–478

Yinuo Wu, Jun Wang, Fei Mao, Fuk Yee Kwong
Palladium-Catalyzed Cross-Dehydrogenative Functionalization of C(sp2)–H Bonds [Focus Review]
Chem. Asian J. 2014, vol. 9, pp. 26–47

Konggang Qu, Jiasi Wang, Jinsong Ren, Xiaogang Qu
Carbon Dots Prepared by Hydrothermal Treatment of Dopamine as an Effective Fluorescent Sensing Platform for the Label-Free Detection of Iron(III) Ions and Dopamine [Full Paper]
Chem. Eur. J. 2013, vol. 19, pp. 7243–7249

Philipp Kaiser, Rajabhau Bajirao Unde, Christoph Kern, Andreas Jess
Production of Liquid Hydrocarbons with CO2 as Carbon Source based on Reverse Water-Gas Shift and Fischer-Tropsch Synthesis [Research Article]
Chem. Ing. Tech. 2013, vol. 85, pp. 489–499

Anthony J. Arduengo, Roland Krafczyk
Auf der Suche nach Stabilen Carbenen [Organische Chemie]
Chem. Unserer Zeit 1998, vol. 32, pp. 6–14

Balayeshwanth R. Vummidi, Jawad Alzeer, Nathan W. Luedtke
Fluorescent Probes for G-Quadruplex Structures [Review]
ChemBioChem 2013, vol. 14, pp. 540–558

Ashish Kumar Singh, Qiang Xu
Synergistic Catalysis over Bimetallic Alloy Nanoparticles [Review]
ChemCatChem 2013, vol. 5, pp. 652–676

Xiaosi Zhou, Yu-Guo Guo
Highly Disordered Carbon as a Superior Anode Material for Room-Temperature Sodium-Ion Batteries [Communication]
ChemElectroChem 2014, vol. 1, pp. 83–86

Marc Steinmetz, Stefan Grimme
Benchmark Study of the Performance of Density Functional Theory for Bond Activations with (Ni,Pd)-Based Transition-Metal Catalysts [Full Paper]
ChemistryOpen 2013, vol. 2, pp. 115–124

Lluís Ballell, Robert H. Bates, Rob J. Young, Daniel Alvarez-Gomez, Emilio Alvarez-Ruiz, Vanessa Barroso, Delia Blanco, Benigno Crespo, Jaime Escribano, Rubén González, Sonia Lozano, Sophie Huss, Angel Santos-Villarejo, José Julio Martín-Plaza, Alfonso Mendoza, María José Rebollo-Lopez, Modesto Remuiñan-Blanco, José Luis Lavandera, Esther Pérez-Herran, Francisco Javier Gamo-Benito, José Francisco García-Bustos, David Barros, Julia P. Castro, Nicholas Cammack
Fueling Open-Source Drug Discovery: 177 Small-Molecule Leads against Tuberculosis [Full Paper]
ChemMedChem 2013, vol. 8, pp. 313–321

Peter Politzer, Jane S. Murray
Halogen Bonding: An Interim Discussion [Review]
ChemPhysChem 2013, vol. 14, pp. 278–294

Philipp Scharf, Jens Müller
Nucleic Acids With Metal-Mediated Base Pairs and Their Applications [Review]
ChemPlusChem 2013, vol. 78, pp. 20–34

Volker Hessel, Dana Kralisch, Norbert Kockmann, Timothy Noël, Qi Wang
Novel Process Windows for Enabling, Accelerating, and Uplifting Flow Chemistry [Review]
ChemSusChem 2013, vol. 6, pp. 746–789

Helena J. Shepherd, Gábor Molnár, William Nicolazzi, Lionel Salmon, Azzedine Bousseksou
Spin Crossover at the Nanometre Scale [Microreview]
Eur. J. Inorg. Chem. 2013, pp. 653–661

Junichiro Yamaguchi, Kei Muto, Kenichiro Itami
Recent Progress in Nickel-Catalyzed Biaryl Coupling [Microreview]
Eur. J. Org. Chem. 2013, pp. 19–30

David Schweinfurth, Naina Deibel, Fritz Weisser, Biprajit Sarkar
Mit Klick zu neuen Liganden [Magazin]
Nachr. Chem. 2011, vol. 59, pp. 937–941
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