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ChemMedChem

Caveat Usor: Assessing Differences between Major Chemistry Databases

Published: 23 February 2018

Author(s): Christopher Southan

Abstract The three databases of PubChem, ChemSpider, and UniChem capture the majority of open chemical structure records with February 2018 totals of 95, 63, and 154 million, respectively. Collectively, they constitute a massively enabling resource for cheminformatics, chemical biology, and drug discovery. As meta‐portals, they subsume and link out to the major proportion of public bioactivity data extracted from the literature and...

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ChemBioChem

A Modular Nanoswitch for Mix‐and‐Detect Protein Assay Based on Binding‐Induced Cascade Dissociation of Kissing Complex

Published: 22 February 2018

Author(s): Yishen Tian, Shanshan Zhang, Li Wang, Shufeng Liu

Abstract A new modular nanoswitch was described for versatile, rapid (within 1 h), homogeneous, and sensitive protein detection. The system employs two hairpins (HP1 and HP2) that can be reciprocally recognized through the apical loop–loop interaction. HP2 possesses a conformation‐switching stem–loop structure, with appended single‐stranded tails on each end, which can hybridize with the recognition‐element‐conjugated DNA strands to...

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ChemCatChem

In Situ Synthesis of Bi 2 O 3 Nanoparticles on ZincMe (Me=Al or Cr) Layered Double Hydroxide Frameworks for Photocatalytic Oxygen Evolution from Water under Solar‐Light Activation

Published: 22 February 2018

Author(s): Gabriela Carja, Diana Gilea, Pegie Cool, Elena M. Seftel

Abstract A key target to boost solar‐to‐chemical conversion processes is to fabricate an efficient solar‐light‐responsive photocatalyst. Herein, we report the in situ synthesis of nanoparticles (NPs) of Bi2O3 directly on Zn‐based layered double hydroxide (LDHs) frameworks. The in situ synthesis of Bi2O3NPs is done at room temperature, is ligand free and explores the ability of calcined ZnMeLDHs to reconstruct their layered structures in Bi(NO3)3 aqueous...

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ChemCatChem

Mechanistic Aspects of Acrylic Acid Formation from CO 2 –Ethylene Coupling over Palladium‐ and Nickel‐based Catalysts

Published: 22 February 2018

Author(s): Yuanhui Li, Zhen Liu, Ruihua Cheng, Boping Liu

Abstract The detailed mechanism of catalytic conversion of CO2 and ethylene to acrylic acid has been investigated through DFT and DLPNO‐CCSD(T) calculations. Four bidentate ligands, dmpe (1,2‐bis(dimethylphosphino)ethane), dcpe (1,2‐bis(dicyclohexylphosphino)ethane), dtbpe (1,2‐bis(di‐tert‐butylphosphino)ethane), and tmeda (tetramethylethylenediamine) were systematically studied to understand the different catalytic behavior of the Pd‐based...

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ChemCatChem

Understanding the Hydro‐Metathesis Reaction of 1‐Decene By Using Well‐Defined Silica Supported W, Mo, Ta Carbene/Carbyne Complexes

Published: 22 February 2018

Author(s): Aya Saidi, Manoja K. Samantaray, Mykyta Tretiakov, Santosh Kavitake, Jean‐Marie Basset

Abstract Direct conversion of 1‐decene to petroleum range alkanes was obtained using hydro‐metathesis reaction. To understand this reaction we employed three different well‐defined single site catalysts precursors; [(≡Si‐O‐)W(CH3)5] 1, [(≡Si‐O‐)Mo(≡CtBu)(CH2tBu)2] 2 and [(≡Si‐O)Ta(=CHtBu)(CH2tBu)2] 3. We witnessed that in our conditions olefin metathesis/isomerization of 1‐decene occurs much faster followed by reduction of the newly formed...

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Chemistry - A European Journal

Reaction Pathway Dependence in Plasmonic Catalysis: Hydrogenation as a Model Molecular Transformation

Published: 22 February 2018

Author(s): Eduardo C. M. Barbosa, Jhonatan L. Fiorio, Tong Mou, Bin Wang, Liane M. Rossi, Pedro H. C. Camargo

Abstract The localized surface plasmon resonance (LSPR) excitation in plasmonic nanoparticles can enhance or mediate chemical transformations. Increased reaction rates for several reactions have been reported due to this phenomenon; however, the fundamental understanding of mechanisms and factors that affect activities remains limited. Here, by investigating hydrogenation reactions as a model transformation and employing different...

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Chemistry - A European Journal

Secondary Metabolites from Escovopsis weberi and Their Role in Attacking the Garden Fungus of Leaf‐Cutting Ants

Published: 22 February 2018

Author(s): Basanta Dhodary, Michele Schilg, Rainer Wirth, Dieter Spiteller

Abstract The specialized, fungal pathogen Escovopsis weberi threatens the mutualistic symbiosis between leaf‐cutting ants and their garden fungus (Leucoagaricus gongylophorus). Because E. weberi can overwhelm L. gongylophorus without direct contact, it was suspected to secrete toxins. Using NMR and mass spectrometry, we identified several secondary metabolites produced by E. weberi. E. weberi produces five shearinine‐type indole triterpenoids including two...

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Chemistry - A European Journal

The Dynamic Equilibrium of Hexakispentafluoroethyldistannane Adducts XSnC 2 F 5 3 SnC 2 F 5 3 XCl Br I SnC 2 F 5 3

Published: 21 February 2018

Author(s): Markus Wiesemann, Johannes Klösener, Beate Neumann, Hans‐Georg Stammler, Berthold Hoge

Abstract The tin–tin bond cleavage of hexaorganodistannanes by nucleophiles is a long‐known reaction and widely used for stannate formation or stannyl group transfer. Herein, we detail our experiments to provide analytical evidence for the existence of the reasonably stable anionic complexes [XSn(C2F5)3{Sn(C2F5)3}]− (X=Cl, Br, I, Sn(C2F5)3) derived from hexakis(pentafluoroethyl)distannane. NMR investigations at low temperature lend further...

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Chemistry - A European Journal

New WaterSoluble Cluster Compound Znen 3 3 V 15 Sb 6 O 42 H 2 O Ethylenediamine 3 10H 2 O as a Synthon for the Generation of Two New Antimonato Polyoxovanadates

Published: 21 February 2018

Author(s): Lisa K. Mahnke, Ulrike Warzok, Mengxi Lin, Christian Näther, Christoph A. Schalley, Wolfgang Bensch

Abstract A new antimonato polyoxovanadate {Zn(en)3}3[V15Sb6O42(H2O)]⋅3 en⋅10 H2O (en=ethylenediamine) synthesized under hydrothermal conditions exhibits remarkable solubility in water. Electrospray ionization mass spectrometry (ESI‐MS) investigations on an aqueous solution demonstrate that the cluster core remains fully intact for 72 h. At longer times, slow transformation into a {V14Sb8O42} cluster is observed. The conversion reaches 50 %...

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Chemistry - A European Journal

Cyclodextrin‐Sandwiched Hexaphyrin Hybrids: Side‐to‐Side Cavity Coupling Switched by a Temperature‐ and Redox‐Responsive Central Device

Published: 21 February 2018

Author(s): Mickaël Ménand, Matthieu Sollogoub, Bernard Boitrel, Stéphane Le Gac

Abstract Access to allosteric enzyme mimics that ideally associate communicating compartments for catalysis and regulation is still challenging. Whereas a sandwich “cavity–catalyst–cavity” approach, developed mainly with cyclodextrins and porphyrins, appears promising, its counterpart with hexaphyrins featuring rich conformation, aromaticity, and coordination behavior has not been prospected at all. We thus developed sandwich...

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Most-accessed articles from each ChemPubSoc Europe, ACES, and GDCh journal

January 2018

 


New Academicians and Foreign Members of the Chinese Academy of Sciences [News]
Angew. Chem. Int. Ed. 2018, vol. 57, p. 1445

Michael Dirkmann, Javier Iglesias-Fernández, Victor Muñoz, Pandian Sokkar, Christoph Rumancev, Andreas von Gundlach, Oktavian Krenczyk, Tobias Vöpel, Julia Nowack, Martin A. Schroer, Simon Ebbinghaus, Christian Herrmann, Axel Rosenhahn, Elsa Sanchez-Garcia, Frank Schulz
A Multiperspective Approach to Solvent Regulation of Enzymatic Activity: HMG-CoA Reductase [Communication]
ChemBioChem 2018, vol. 19, p. 153

Isabela C. Man, Hai-Yan Su, Federico Calle-Vallejo, Heine A. Hansen, José I. Martínez, Nilay G. Inoglu, John Kitchin, Thomas F. Jaramillo, Jens K. Nørskov, Jan Rossmeisl
Universality in Oxygen Evolution Electrocatalysis on Oxide Surfaces [Full Paper]
ChemCatChem 2011, vol. 3, p. 1159

Matthias Ducci
Geheimtinten [Artikel]
Chem. Unserer Zeit 2017, vol. 51, p. 228

Balaram Mukhopadhyay, Rituparna Das
Chemical O-Glycosylations: An Overview [Review]
ChemistryOpen 2016, vol. 5, p. 401

Lei Han, Meng-Ke Wu, Fei-Yan Yi, Dongxiao Chen, Hai-Long Jiang
Chemical Sensors Based on Metal-Organic Frameworks [Review]
ChemPlusChem 2016, vol. 81, p. 675

Miaofang Chi, Harry M. Meyer, Zili Wu, Liangbo Liang, Peter V. Bonnesen, Dale K. Hensley, Rui Peng, Yang Song, Cheng Ma, Bobby G. Sumpter, Adam J. Rondinone
High-Selectivity Electrochemical Conversion of CO2 to Ethanol using a Copper Nanoparticle/N-Doped Graphene Electrode [Full Paper]
ChemistrySelect 2016, vol. 1, p. 6055

Ekkehard Schwab, Sebastian Schiebahn, Georg Schaub, Martin Reuter, Konstantin Räuchle, Ludolf Plass, Marcell Peuckert, Anja Metzelthin, Falko Mahlendorf, Wolfram Koch, Renate Hoer, Angelika Heinzel, Sigmar Bräuninger, Martin Bertau, Christian Beilmann, Florian Ausfelder, Ferdi Schüth, Detlef Stolten, Gisa Teßmer, Kurt Wagemann, Karl-Friedrich Ziegahn
Energiespeicherung als Element einer sicheren Energieversorgung [Übersichtsbeitrag]
Chem. Ing. Tech. 2015, vol. 87, p. 17

Abas Mohsenzadeh, Akram Zamani, Mohammad J. Taherzadeh
Bioethylene Production from Ethanol: A Review and Techno-economical Evaluation [Review]
ChemBioEng Rev. 2017, vol. 4, p. 75

Lantao Liu, Yanli Zhou, Shuang Liu, Maotian Xu
The Applications of Metal−Organic Frameworks in Electrochemical Sensors [Review]
ChemElectroChem 2018, vol. 5, p. 6

Yinghui Xue, Qin Zhang, Tao Zhang, Lei Fu
Black Phosphorus: Properties, Synthesis, and Applications in Energy Conversion and Storage [Focus Review]
ChemNanoMat 2017, vol. 3, p. 352

Haymo Ross
We are Family (Chemistry Smash Hits) [Editorial]
Chem. Eur. J. 2018, vol. 24, p. 6

Xinzhe Shi, Arpan Sasmal, Jean-François Soulé, Henri Doucet
Metal-Catalyzed C−H Bond Activation of 5-Membered Carbocyclic Rings: A Powerful Access to Azulene, Acenaphthylene and Fulvene Derivatives [Focus Review]
Chem. Asian J. 2018, vol. 13, p. 143

Andrea Gualandi, Luca Mengozzi, Pier Giorgio Cozzi
Iron-Promoted Radical Reactions: Current Status and Perspectives [Focus Review]
Asian J. Org. Chem. 2017, vol. 6, p. 1160

Truong-Thanh Tung, Trong T. Dao, Marta G. Junyent, Michael Palmgren, Thomas Günther-Pomorski, Anja T. Fuglsang, Søren B. Christensen, John Nielsen
Cover Feature: LEGO-Inspired Drug Design: Unveiling a Class of Benzo[d]thiazoles Containing a 3,4-Dihydroxyphenyl Moiety as Plasma Membrane H+-ATPase Inhibitors (ChemMedChem 1/2018) [Cover Picture]
ChemMedChem 2018, vol. 13, p. 2

Zhoufeng Bian, Sonali Das, Ming Hui Wai, Plaifa Hongmanorom, Sibudjing Kawi
A Review on Bimetallic Nickel-Based Catalysts for CO2 Reforming of Methane [Review]
ChemPhysChem 2017, vol. 18, p. 3117

Dogukan Hazar Apaydin, Dong Ryeol Whang
Artificial Photosynthesis: Learning from Nature [Review]
ChemPhotoChem 10.1002/cptc.201700163

Jiwhan Kim, Hee-Eun Kim, Hyunjoo Lee
Single-Atom Catalysts of Precious Metals for Electrochemical Reactions [Minireview]
ChemSusChem 2018, vol. 11, p. 104

Ross J. Marshall, Ross S. Forgan
Postsynthetic Modification of Zirconium Metal-Organic Frameworks [Microreview]
Eur. J. Inorg. Chem. 2016, p. 4310

Davin Tan, Tomislav Friščić
Mechanochemistry for Organic Chemists: An Update [Microreview]
Eur. J. Org. Chem. 2018, p. 18

Deutscher Lebensmittelchemikertag 2016 in Freising-Weihenstephan [Vorträge]
Lebensmittelchemie 2017, vol. 71, p. 2

Meilensteine der Chemie 2018 [Bildung & Gesellschaft]
Nachr. Chem. 2018, vol. 66, p. 38

Katrin Sommer, Christina Toschka, Laura Schröder, Thomas Philipp Schröder, Henning Steff, Roland A. Fischer
Modellexperimente im Chemieunterricht. [Artikel]
CHEMKON 2017, vol. 24, p. 13

Catharina Goedecke
Why Does Iodine Turn Starch Blue?
ChemViews Magazine 2016

Most cited articles from each ChemPubSoc Europe, ACES, and GDCh journal


2016

 


Shoujun Zhu, Qingnan Meng, Lei Wang, Junhu Zhang, Yubin Song, Han Jin, Kai Zhang, Hongchen Sun, Haiyu Wang, Bai Yang
Highly Photoluminescent Carbon Dots for Multicolor Patterning, Sensors, and Bioimaging
Angew. Chem. Int. Ed. 2013, vol. 52, pp. 3953–3957

Balayeshwanth R. Vummidi, Jawad Alzeer, Nathan W. Luedtke
Fluorescent Probes for G-Quadruplex Structures [Review]
ChemBioChem 2013, vol. 14, pp. 540–558

Zhi-Yuan Gu, Jihye Park, Aaron Raiff, Zhangwen Wei, Hong-Cai Zhou
Metal–Organic Frameworks as Biomimetic Catalysts [Minireview]
ChemCatChem 2014, vol. 6, pp. 67–75

Anthony J. Arduengo, Roland Krafczyk
Auf der Suche nach Stabilen Carbenen [Organische Chemie]
Chem. Unserer Zeit 1998, vol. 32, pp. 6–14

Marc Steinmetz, Stefan Grimme
Benchmark Study of the Performance of Density Functional Theory for Bond Activations with (Ni,Pd)-Based Transition-Metal Catalysts [Full Paper]
ChemistryOpen 2013, vol. 2, pp. 115–124

Philipp Scharf, Jens Müller
Nucleic Acids With Metal-Mediated Base Pairs and Their Applications [Review]
ChemPlusChem 2013, vol. 78, pp. 20–34

Philipp Kaiser, Rajabhau Bajirao Unde, Christoph Kern, Andreas Jess
Production of Liquid Hydrocarbons with CO2 as Carbon Source based on Reverse Water-Gas Shift and Fischer-Tropsch Synthesis [Research Article]
Chem. Ing. Tech. 2013, vol. 85, pp. 489–499

Xiaosi Zhou, Yu-Guo Guo
Highly Disordered Carbon as a Superior Anode Material for Room-Temperature Sodium-Ion Batteries [Communication]
ChemElectroChem 2014, vol. 1, pp. 83–86

Chuanxi Wang, Zhenzhu Xu, Chi Zhang
Polyethyleneimine-Functionalized Fluorescent Carbon Dots: Water Stability, pH Sensing, and Cellular Imaging [Full Paper]
ChemNanoMat 2015, vol. 1, pp. 122–127

Konggang Qu, Jiasi Wang, Jinsong Ren, Xiaogang Qu
Carbon Dots Prepared by Hydrothermal Treatment of Dopamine as an Effective Fluorescent Sensing Platform for the Label-Free Detection of Iron(III) Ions and Dopamine [Full Paper]
Chem. Eur. J. 2013, vol. 19, pp. 7243–7249

Yinuo Wu, Jun Wang, Fei Mao, Fuk Yee Kwong
Palladium-Catalyzed Cross-Dehydrogenative Functionalization of C(sp2)–H Bonds [Focus Review]
Chem. Asian J. 2014, vol. 9, pp. 26–47

Naohiko Yoshikai, Ye Wei
Synthesis of Pyrroles, Indoles, and Carbazoles through Transition-Metal-Catalyzed C–H Functionalization [Review]
Asian J. Org. Chem. 2013, vol. 2, pp. 466–478

Lluís Ballell, Robert H. Bates, Rob J. Young, Daniel Alvarez-Gomez, Emilio Alvarez-Ruiz, Vanessa Barroso, Delia Blanco, Benigno Crespo, Jaime Escribano, Rubén González, Sonia Lozano, Sophie Huss, Angel Santos-Villarejo, José Julio Martín-Plaza, Alfonso Mendoza, María José Rebollo-Lopez, Modesto Remuiñan-Blanco, José Luis Lavandera, Esther Pérez-Herran, Francisco Javier Gamo-Benito, José Francisco García-Bustos, David Barros, Julia P. Castro, Nicholas Cammack
Fueling Open-Source Drug Discovery: 177 Small-Molecule Leads against Tuberculosis [Full Paper]
ChemMedChem 2013, vol. 8, pp. 313–321

Peter Politzer, Jane S. Murray
Halogen Bonding: An Interim Discussion [Review]
ChemPhysChem 2013, vol. 14, pp. 278–294

Volker Hessel, Dana Kralisch, Norbert Kockmann, Timothy Noël, Qi Wang
Novel Process Windows for Enabling, Accelerating, and Uplifting Flow Chemistry [Review]
ChemSusChem 2013, vol. 6, pp. 746–789

Helena J. Shepherd, Gábor Molnár, William Nicolazzi, Lionel Salmon, Azzedine Bousseksou
Spin Crossover at the Nanometre Scale [Microreview]
Eur. J. Inorg. Chem. 2013, pp. 653–661

Junichiro Yamaguchi, Kei Muto, Kenichiro Itami
Recent Progress in Nickel-Catalyzed Biaryl Coupling [Microreview]
Eur. J. Org. Chem. 2013, pp. 19–30

David Schweinfurth, Naina Deibel, Fritz Weisser, Biprajit Sarkar
Mit Klick zu neuen Liganden [Magazin]
Nachr. Chem. 2011, vol. 59, pp. 937–941
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