Graphene-MoS2 Heterostructures for Solid-State Lasers

  • Author: Liam Critchley
  • Published: 13 November 2018
  • Copyright: Wiley-VCH Verlag GmbH & Co. KGaA
  • Source / Publisher: ACS Nano/ACS Publications
  • Associated Societies: American Chemical Society (ACS), USA
thumbnail image: Graphene-MoS<sub>2</sub> Heterostructures for Solid-State Lasers

2D materials such as graphene and transition metal dichalcogenides (TMDCs) can be layered together in many configurations to create van-der-Waals (vdW) heterostructures. Within these heterostructures, the optical and electrical properties are influenced by interlayer coupling. Because graphene and MoS2 have complementary properties, vdW heterostructures composed of these two materials have been shown to be useful for optoelectronic devices.

Baitao Zhang, Yanlu Li, and colleagues, Shandong University, China, have used density functional theory (DFT) calculations to find the theoretical optimal thickness and layering of a graphene-MoS2 heterostructure for use in lasers. The layer thickness influences the interlayer coupling. The team then synthesized the heterostructures using chemical vapor deposition (CVD) and used them as saturable absorbers in a femtosecond solid-state laser.

The researchers found that heterostructures composed of one to four layers of MoS2 were the most efficient. The thickness of MoS2 in the heterostructure affects the nonlinear optical response. The prepared vdW heterostructures have work functions between 4.63 and 5.00 eV. When the heterostructures were incorporated into a laser, it achieved pulses as short as 236 fs and an output power of 0.55 W. According to the researchers, these are the best results ever achieved with a heterostructure-based mode-locked laser.


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