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Nitrogen‐Doped Carbons with Hierarchical Porosity via Chemical Blowing Towards Long‐Lived Metal‐Free Catalysts for Acetylene Hydrochlorination

Published: 17 January 2020

Author(s): Selina K. Kaiser, Kyung Seob Song, Sharon Mitchell, Ali Coskun, Javier Pérez‐Ramírez

Abstract Porous nitrogen‐doped carbons (NCs) are sustainable alternatives to the toxic mercury‐based acetylene hydrochlorination catalysts applied in the manufacture of polyvinyl chloride. However, the application of NCs as metal‐free catalysts is hampered by their insufficient durability under industrially relevant process conditions. In particular, pore blockage leads to accelerated deactivation of NCs compared to the state‐of‐the‐art precious metal‐based systems. Herein, we develop a salt...

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Catalytic Transfer Hydrogenation of Furfural over Co3O4−Al2O3 Hydrotalcite‐derived Catalyst

Published: 17 January 2020

Author(s): Ruben Ramos, Andreia F. Peixoto, Blanca I. Arias‐Serrano, O. Salomé G. P. Soares, Manuel F. R. Pereira, David Kubička, Cristina Freire

Abstract The hydrogenation of furfural by catalytic hydrogen transfer to produce furfuryl alcohol has been investigated over a series of mixed oxides derived from hydrotalcite catalysts. Three different catalysts containing Ni, Co and Zn phases on an Al‐rich amorphous support were synthesized and characterised. The catalytic performances were evaluated in a batch stirred reactor using 2‐propanol as a solvent and hydrogen donor, with Co3O4−Al2O3 showing the highest activity and selectivity to...

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A Novel Earth‐Abundant W‐WC Heterojunction as Efficient Co‐Catalyst for Enhanced Photocatalytic H2 Evolution

Published: 17 January 2020

Author(s): Baojun Ma, Sipeng Zhang, Wei Wang, Li Feng, Ruisheng Zhang, Keying Lin, Dekang Li, Haijuan Zhan, Xu Yang

Abstract New functional materials are of significance for the industry development of coal and tungsten. Here, we reported a novel earth‐abundant W‐WC heterojunction on CdS as an efficient and cheap co‐catalyst for photocatalytic H2 evolution on CdS under visible light irradiation. The W‐WC is simply synthesized from industrial raw material of coal and ammonium tungstate by a simple one‐step calcination strategy. The photocatalytic activities tests show that W‐WC heterojunction has better...

thumbnail image: ChemCatChem


3D‐Graphene Decorated with g‐C3N4/Cu3P Composite: A Noble Metal‐free Bifunctional Electrocatalyst for Overall Water Splitting

Published: 17 January 2020

Author(s): Sk. Riyajuddin, S. K. Tarik Aziz, Sushil Kumar, Gilbert D. Nessim, Kaushik Ghosh

Abstract Electrochemical water splitting, which generates both hydrogen and oxygen, using highly efficient and low‐cost noble metal‐free (Pt, Ru, Ir etc.) electrocatalyst is an economical and green approach for the alternative energy source. Due to their conductivity, durability and long‐term stability, carbonaceous containing hybrid materials are used as promising electrodes for total water splitting. Herein, the design of metal‐phosphide (Cu3P) with graphitic carbon‐nitride (g‐C3N4)...

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Theoretical Study of Rhodium‐Catalyzed C−C Activation of Cyclobutanones: Origin of Ligand‐Controlled Product Selectivity

Published: 17 January 2020

Author(s): Tian Zhang, Xiajun Wu, Juan Li

Abstract Cyclobutanone C−C activation with a Rh(I) catalyst has great potential for the synthesis of fused‐ and bridged‐ring systems. However, this synthetic application is greatly limited because of the direct CO extrusion from cyclobutanone, which leads to formation of cyclopropane as a byproduct. The calculations rationalize the experimental puzzles: why PMe2Ph and XPhos ligands can prevent cyclopropane formation for C2‐ and C3‐substituted cyclobutanone, respectively. More importantly, we...

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Metal‐Organic Sheets for Efficient Drug Delivery and Bioimaging

Published: 17 January 2020

Author(s): Yucong Song, Jingjie Yang, Lei Wang, Zhigang Xie

Abstract Metal‐organic frameworks (MOFs) formed by coordination between metal ions or clusters and organic bridging ligands possess great potential for biomedicine applications, given their high biocompatibility and biodegradability. Compared with the traditional three‐dimensional (3D) MOFs, two‐dimensional (2D) MOFs with sheet‐like morphologies exhibit unique properties. In this study, a nanoscale 2D leaf‐shaped MOF (NZIF−L) was synthesized via coordination self‐assembly between...

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Protein Therapeutics. Edited by Tristan Vaughan, Jane Osbourn, and Bahija Jallal

Published: 17 January 2020

Author(s): Seah Ling Kuan

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Kemp Elimination Reaction Catalyzed by Electric Fields

Published: 17 January 2020

Author(s): Carles Acosta‐Silva, Joan Bertran, Vicenç Branchadell, Antoni Oliva

Abstract The Kemp elimination reaction is the most widely used in the de novo design of new enzymes. The effect of two different kinds of electric fields in the reactions of acetate as a base with benzisoxazole and 5‐nitrobenzisoxazole as substrates have been theoretically studied. The effect of the solvent reaction field has been calculated using the SMD continuum model for several solvents; we have shown that solvents inhibit both reactions, the decrease of the reaction rate being larger as...

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Chemistry - A European Journal

Bioluminescence Profiling of NanoKAZ/NanoLuc Luciferase Using a Chemical Library of Coelenterazine Analogues

Published: 17 January 2020

Author(s): Eloi P. Coutant, Glwadys Gagnot, Vincent Hervin, Racha Baatallah, Sophie Goyard, Yves Jacob, Thierry Rose, Yves L. Janin

Abstract We describe here an extensive structure‐bioluminescence relationship study of a chemical library of analogues of coelenterazine, using nanoKAZ/NanoLuc, a mutated luciferase originated from the catalytic subunit of the deep‐sea shrimp Oplophorus gracilirostris. Out of the 135 O‐acetylated precursors that were prepared by using our recently reported synthesis and following their hydrolysis to give solutions of the corresponding luciferins, notable bioluminescence improvements were...

thumbnail image: Chemistry - A European Journal

Chemistry - A European Journal

Hetero Diels–Alder Reactions of Masked Dienes Containing Heavy Group 15 Elements

Published: 17 January 2020

Author(s): Monika Kořenková, Vít Kremláček, Martin Hejda, Jan Turek, Raffi Khudaverdyan, Milan Erben, Roman Jambor, Aleš Růžička, Libor Dostál

Abstract Treatment of N,C,N‐chelated organopnictogen(I) compounds ArE (1–3) (Ar=2,6‐(RN=CH)2C6H3, E/R=As/Dmp (1), Sb/tBu (2), and Bi/tBu (3), where Dmp=2,6‐Me2C6H3) with various electron‐deficient alkynes RC≡CR′ (R/R′=CO2Me (DMAD), R/R′=H/CO2Me, or R/R′=NC5F4) affords different types of heterocyclic compounds. In these reactions, 1–3 act as hidden dienes and participate in hetero‐Diels–Alder (DA) reactions, a feature that has been only rarely reported for heavier pnictogen compounds. In this...

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Most-accessed articles from each ChemPubSoc Europe, ACES, and GDCh journal

December 2019


Duanyang Kong, Patrick J. Moon, Odey Bsharat, Rylan J. Lundgren
Direct Catalytic Decarboxylative Amination of Aryl Acetic Acids [Research Article]
Angew. Chem. Int. Ed. 2020, vol. 59, no. 3, p. 1313

Bing Liu, Lihui He, Liping Wang, Tao Li, Changcheng Li, Huayi Liu, Yunzi Luo, Rui Bao
Protein Crystallography and Site-Direct Mutagenesis Analysis of the Poly(ethylene terephthalate) Hydrolase PETase from Ideonella sakaiensis [Communication]
ChemBioChem 2018, vol. 19, no. 14, p. 1471

Isabela C. Man, Hai-Yan Su, Federico Calle-Vallejo, Heine A. Hansen, José I. Martínez, Nilay G. Inoglu, John Kitchin, Thomas F. Jaramillo, Jens K. Nørskov, Jan Rossmeisl
Universality in Oxygen Evolution Electrocatalysis on Oxide Surfaces [Full Paper]
ChemCatChem 2011, vol. 3, no. 7, p. 1159

Wolfgang Pfeiffer, Van Than Nguyen, Jan Neumann, Dirk Awe, Jens Tränckner
Operation and Control of a Full-Scale Biogas Plant Treating Wastewater from the Cleaning of Car Tanks [Research Article]
Chem. Eng. Technol. 2020, vol. 43, no. 1, p. 84

Dieter Wöhrle
Kunststoffe [Artikel]
Chem. Unserer Zeit 2019, vol. 53, no. 1, p. 50

Luling Wu, Xue Tian, Hai-Hao Han, Jie Wang, Robin R. Groleau, Paramabhorn Tosuwan, Boontana Wannalerse, Adam C. Sedgwick, Steven D. Bull, Xiao-Peng He, Tony D. James
A Simple Near-Infrared Fluorescent Probe for the Detection of Peroxynitrite [Communication]
ChemistryOpen 2019, vol. 8, no. 12, p. 1407

Daewoo Han, Andrew J. Steckl
Coaxial Electrospinning Formation of Complex Polymer Fibers and their Applications [Review]
ChemPlusChem 2019, vol. 84, no. 10, p. 1453

Miaofang Chi, Harry M. Meyer, Zili Wu, Liangbo Liang, Peter V. Bonnesen, Dale K. Hensley, Rui Peng, Yang Song, Cheng Ma, Bobby G. Sumpter, Adam J. Rondinone
High-Selectivity Electrochemical Conversion of CO2 to Ethanol using a Copper Nanoparticle/N-Doped Graphene Electrode [Full Paper]
ChemistrySelect 2016, vol. 1, no. 19, p. 6055

Ekkehard Schwab, Sebastian Schiebahn, Georg Schaub, Martin Reuter, Konstantin Räuchle, Ludolf Plass, Marcell Peuckert, Anja Metzelthin, Falko Mahlendorf, Wolfram Koch, Renate Hoer, Angelika Heinzel, Sigmar Bräuninger, Martin Bertau, Christian Beilmann, Florian Ausfelder, Ferdi Schüth, Detlef Stolten, Gisa Teßmer, Kurt Wagemann, Karl-Friedrich Ziegahn
Energiespeicherung als Element einer sicheren Energieversorgung [Übersichtsbeitrag]
Chem. Ing. Tech. 2015, vol. 87, no. 1-2, p. 17

Abas Mohsenzadeh, Akram Zamani, Mohammad J. Taherzadeh
Bioethylene Production from Ethanol: A Review and Techno-economical Evaluation [Review]
ChemBioEng Rev. 2017, vol. 4, no. 2, p. 75

Lucia Mazzapioda, Carmelo Lo Vecchio, Annalisa Paolone, Antonino Salvatore Aricò, Vincenzo Baglio, Maria Assunta Navarra
Enhancing Oxygen Reduction Reaction Catalytic Activity Using a Sub-Stoichiometric CaTiO3−δ Additive [Cover Profile]
ChemElectrochem 2019, vol. 6, no. 24, p. 5910

S. Ghosh, B. Pradhan
Lead-Free Metal Halide Perovskite Nanocrystals: Challenges, Applications, and Future Aspects [Minireview]
ChemNanoMat 2019, vol. 5, no. 3, p. 300

Frank Tabellion, Christoph Peters, Uwe Fischbeck, Manfred Regitz, Fritz Preuss
Imidovanadium(V) Complexes as Reaction Partners for Kinetically Stabilized Phosphaalkynes: Synthesis of 1,2,4‐Azaphosphavanada(V)‐cyclobutenes, 1,3,5‐Triphosphabenzenes, and 1H‐1,2,4‐Azadiphospholes [Organophosphorus Compounds, Part 148 : Full Paper]
Chem. Eur. J. 2000, vol. 6, no. 24, p. 4558

Byunghyuck Jung, Jungkyu K. Lee, Jungnam Kim, Eunhye K. Kang, Sang Yeong Han, Hee-Yoon Lee, Insung S. Choi
Synthetic Strategies for (−)-Cannabidiol and Its Structural Analogs [Minireview]
Chem. Asian J. 2019, vol. 14, no. 21, p. 3749

Arun K. Sinha, Danish Equbal
Thiol−Ene Reaction: Synthetic Aspects and Mechanistic Studies of an Anti-Markovnikov-Selective Hydrothiolation of Olefins [Focus Review]
Asian J. Org. Chem. 2019, vol. 8, no. 1, p. 32

Avick Kumar Ghosh, Indranil Samanta, Anushree Mondal, Wenshe Ray Liu
Covalent Inhibition in Drug Discovery [Review]
ChemMedChem 2019, vol. 14, no. 9, p. 889

Andrea Álvarez, Marta Borges, Juan José Corral-Pérez, Joan Giner Olcina, Lingjun Hu, Damien Cornu, Rui Huang, Dragos Stoian, Atsushi Urakawa
CO2 Activation over Catalytic Surfaces [Concept]
ChemPhysChem 2017, vol. 18, no. 22, p. 3135

Matthias Freitag, Nadja Möller, Andreas Rühling, Cristian A. Strassert, Bart Jan Ravoo, Frank Glorius
Photocatalysis in the Dark: Near-Infrared Light Driven Photoredox Catalysis by an Upconversion Nanoparticle/Photocatalyst System [Communication]
ChemPhotoChem 2019, vol. 3, no. 1, p. 24

Mingshuai Ma, Lin Dai, Chuanling Si, Lanfeng Hui, Zhong Liu, Yonghao Ni
Front Cover: A Facile Preparation of Super Long-Term Stable Lignin Nanoparticles from Black Liquor (ChemSusChem 24/2019) [Cover Picture]
ChemSusChem 2019, vol. 12, no. 24, p. 5213

Stephen A. Matlin, Goverdhan Mehta, Henning Hopf, Alain Krief
The Periodic Table of the Chemical Elements and Sustainable Development [Essay]
Eur. J. Inorg. Chem. 2019, p. 4170

Luca Capaldo, Davide Ravelli
Hydrogen Atom Transfer (HAT): A Versatile Strategy for Substrate Activation in Photocatalyzed Organic Synthesis [Microreview]
Eur. J. Org. Chem. 2017, p. 2056

Cover Picture Lebensmittelchemie 6/2019 [Cover Picture]
Lebensmittelchemie 2019, vol. 73, no. 6

Elementerätsel 1 [Wissenschaft + Forschung]
Nachr. Chem. 2019, vol. 67, no. 12, p. 40

Schüleraufgabe: CHEMKON 2/2017 [Schüleraufgabe]
CHEMKON 2017, vol. 24, no. 2, p. 91

Zheng Ma, Douglas R. MacFarlane, Mega Kar
Mg Cathode Materials and Electrolytes for Rechargeable Mg Batteries: A Review [Minireview]
Batteries & Supercaps 2019, vol. 2, no. 2, p. 115

Catharina Goedecke
Why Does Iodine Turn Starch Blue?
ChemViews Magazine 2016

Most cited articles from each ChemPubSoc Europe, ACES, and GDCh journal



Eric J. Popczun, Carlos G. Read, Christopher W. Roske, Nathan S. Lewis, Raymond E. Schaak
Highly Active Electrocatalysis of the Hydrogen Evolution Reaction by Cobalt Phosphide Nanoparticles
Angew. Chem. Int. Ed. 2014, vol. 53, pp. 5427–5430

Philippe Compain, Anne Bodlenner
The Multivalent Effect in Glycosidase Inhibition: A New, Rapidly Emerging Topic in Glycoscience [Minireview]
ChemBioChem 2014, vol. 15, pp. 1239–1251

Zhi-Yuan Gu, Jihye Park, Aaron Raiff, Zhangwen Wei, Hong-Cai Zhou
Metal–Organic Frameworks as Biomimetic Catalysts [Minireview]
ChemCatChem 2014, vol. 6, pp. 67–75

Anthony J. Arduengo, Roland Krafczyk
Auf der Suche nach Stabilen Carbenen [Organische Chemie]
Chem. Unserer Zeit 1998, vol. 32, pp. 6–14

Félix Sancenón, Lluís Pascual, Mar Oroval, Elena Aznar, Ramón Martínez-Máñez
Gated Silica Mesoporous Materials in Sensing Applications [Review]
ChemistryOpen 2015, vol. 4, pp. 418–437

Jun Pu, Tingting Wang, Haiyang Wang, Yao Tong, Chenchen Lu, Wei Kong, Zhenghua Wang
Direct Growth of NiCo2S4 Nanotube Arrays on Nickel Foam as High-Performance Binder-Free Electrodes for Supercapacitors [Full Paper]
ChemPlusChem 2014, vol. 79, pp. 577–583

Francisco Trespalacios, Ignacio E. Grossmann
Review of Mixed-Integer Nonlinear and Generalized Disjunctive Programming Methods [Review]
Chemie Ingenieur Technik 2014, vol. 86, pp. 991–1012

Xiaosi Zhou, Yu-Guo Guo
Highly Disordered Carbon as a Superior Anode Material for Room-Temperature Sodium-Ion Batteries [Communication]
ChemElectroChem 2014, vol. 1, pp. 83–86

Chuanxi Wang, Zhenzhu Xu, Chi Zhang
Polyethyleneimine-Functionalized Fluorescent Carbon Dots: Water Stability, pH Sensing, and Cellular Imaging [Full Paper]
ChemNanoMat 2015, vol. 1, pp. 122–127

Matthew N. Hopkinson, Basudev Sahoo, Jun-Long Li, Frank Glorius
Dual Catalysis Sees the Light: Combining Photoredox with Organo-, Acid, and Transition-Metal Catalysis [Minireview]
Chemistry – A European Journal 2014, vol. 20, pp. 3874–3886

Yinuo Wu, Jun Wang, Fei Mao, Fuk Yee Kwong
Palladium-Catalyzed Cross-Dehydrogenative Functionalization of C(sp2)–H Bonds [Focus Review]
Chemistry – An Asian Journal 2014, vol. 9, pp. 26–47

Derong Cao, Herbert Meier
Pillar[n]arenes—a Novel, Highly Promising Class of Macrocyclic Host Molecules [Focus Review]
Asian Journal of Organic Chemistry 2014, vol. 3, pp. 244–262

Daniel Gallenkamp, Kathy A. Gelato, Bernard Haendler, Hilmar Weinmann
Bromodomains and Their Pharmacological Inhibitors [Review]
ChemMedChem 2014, vol. 9, pp. 438–464

Antonio Bauzá, Tiddo J. Mooibroek, Antonio Frontera
The Bright Future of Unconventional σ/π-Hole Interactions [Review]
ChemPhysChem 2015, vol. 16, pp. 2496–2517

Ksenia S. Egorova, Valentine P. Ananikov
Toxicity of Ionic Liquids: Eco(cyto)activity as Complicated, but Unavoidable Parameter for Task-Specific Optimization [Review]
ChemSusChem 2014, vol. 7, pp. 336–360

Shunichi Fukuzumi, Dachao Hong
Homogeneous versus Heterogeneous Catalysts in Water Oxidation [Microreview]
Eur. J. Inorg. Chem. 2014, pp. 645–659

Fabien Toulgoat, Sébastien Alazet, Thierry Billard
Direct Trifluoromethylthiolation Reactions: The “Renaissance” of an Old Concept [Microreview]
Eur. J. Org. Chem. 2014, pp. 2415–2428

David Schweinfurth, Naina Deibel, Fritz Weisser, Biprajit Sarkar
Mit Klick zu neuen Liganden [Magazin]
Nachr. Chem. 2011, vol. 59, pp. 937–941

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A product of ChemPubSoc Europe (16 European Chemical Societies)published by Wiley-VCH