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Chemistry - A European Journal

Nickel‐Mediated Photoreductive Cross Coupling of Carboxylic Acid Derivatives for Ketone Synthesis**

Published: 23 November 2021

Author(s): Jan Brauer, Elisabeth Quraishi, Lisa Marie Kammer, Till Opatz

Abstract A simple visible light photochemical, nickel‐catalyzed synthesis of ketones from carboxylic acid‐derived precursors is presented. Hantzsch ester (HE) functions as a cheap, green and strong photoreductant to facilitate radical generation and also engages in the Ni‐catalytic cycle to restore the reactive species. With this dual role, HE allows for the coupling of a large variety of radicals (1°,2°, benzylic, α‐oxy & α‐amino) with aroyl and alkanoyl moieties, a new feature in reactions...

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Structure and Photophysical Properties of 1,1,2,2‐Tetra(1‐anthryl)ethane: A C(sp3)−C(sp3) Bond Substituted with Four Anthracene Units

Published: 23 November 2021

Author(s): Shu Aoki, Eiji Tsurumaki, Masahiro Yamashina, Kan Wakamatsu, Shinji Toyota

Abstract The title aromatic compound comprising four anthracene units was synthesized by the McMurry coupling of di(1‐anthryl) ketone as a hydrogenated product in 65 % yield. The molecule forms a C2 symmetric structure with the ap conformation about the C(sp3)−C(sp3) single bond, as revealed by X‐ray analysis and DFT calculations. The UV/vis and fluorescence spectra of this compound were compared with those of anthracene, di(1‐anthryl)methane, and 1,2‐di(1‐anthryl)ethane. The fluorescence...

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N,N‐Dimethylformamide‐protected Fe2O3 Combined with Pt Nanoparticles: Characterization and Catalysis in Alkene Hydrosilylation

Published: 23 November 2021

Author(s): Tatsuki Nagata, Tatsuya Tanaka, Xianjin Lin, Ryota Kondo, Takeyuki Suzuki, Yasuharu Kanda, Takashi Toyao, Ken‐ichi Shimizu, Yasushi Obora

Abstract We report a combination of N,N‐dimethylformamide (DMF)‐protected Fe2O3 nanoparticles (NPs) and Pt NPs for the hydrosilylation of various industrially relevant alkenes and tertiary silanes. The DMF‐protected Fe2O3 and Pt NPs catalysts were characterized by transmission electron microscopy, X‐ray absorption spectroscopy, and X‐ray photoelectron spectroscopy. The catalyst of DMF‐protected Fe2O3 NPs combined with Pt NPs can be recycled for five cycles by a simple extraction using...

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Chemistry - A European Journal

Conversion of E4 (E4=P4, As4, AsP3) by Ni(0) and Ni(I) Synthons – A Comparative Study

Published: 23 November 2021

Author(s): Maria Haimerl, Christian Graßl, Michael Seidl, Martin Piesch, Manfred Scheer

Abstract The reactivity of white phosphorus and yellow arsenic towards two different nickel nacnac complexes is investigated. The nickel complexes [(L1Ni)2tol] (1, L1=[{N(C6H3iPr2‐2,6)C(Me)}2CH]−) and [K2][(L1Ni)2(μ,η1 : 1‐N2)] (6) were reacted with P4, As4 and the interpnictogen compound AsP3, respectively, yielding the homobimetallic complexes [(L1Ni)2(μ‐η2,κ1:η2,κ1‐E4)] (E=P (2 a), As (2 b), AsP3 (2 c)), [(L1Ni)2(μ,η3 : 3‐E3)] (E=P (3 a), As (3 b)) and [[email protected]‐c‐6(thf)2][L1Ni(η1 : 1‐E4)] (E=P...

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Chemistry - A European Journal

Acid‐Catalyzed RNA‐Oligomerization from 3’,5’‐cGMP

Published: 23 November 2021

Author(s): Sreekar Wunnava, Christina F. Dirscherl, Jakub Výravský, Aleš Kovařík, Roman Matyášek, Jiří Šponer, Dieter Braun, Judit E. Šponer

Abstract The assembly of ancient informational polymers from nucleotide precursors is the central challenge of life's origin on our planet. Among the possible solutions, dry polymerization of 3’,5’‐cyclic guanosine monophosphate (3’,5’‐cGMP) has been proposed as a candidate to create oligonucleotides of 15–20 units in length. However, the reported sensitivity of the reaction to the presence of cations raised questions of whether this chemistry could be relevant in a geological context. The...

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Chemistry - A European Journal

Unveiling the Unique Roles of Metal Coordination and Modulator in the Polymorphism Control of Metal‐Organic Frameworks

Published: 23 November 2021

Author(s): Zi‐Jian Li, Yu Ju, Zeya Zhang, Huangjie Lu, Yongxin Li, Ningjin Zhang, Xian‐Long Du, Xiaofeng Guo, Zhi‐Hui Zhang, Yuan Qian, Ming‐Yang He, Jian‐Qiang Wang, Jian Lin

Abstract Polymorphism control of metal‐organic frameworks is highly desired for elucidating structure‐property relationships, but remains an empirical process and is usually done in a trial‐and‐error approach. We adopted the rarely used actinide cation Th4+ and a ditopic linker to construct a series of thorium‐organic frameworks (TOFs) with a range of polymorphs. The extraordinary coordination versatility of Th4+ cations and clusters, coupled with synthetic modulation, gives five distinct...

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Chemistry - A European Journal

Tuning the Reactivity of a Substrate for SNAP‐Tag Expands Its Application for Recognition‐Driven DNA‐Protein Conjugation

Published: 23 November 2021

Author(s): Zhengxiao Zhang, Eiji Nakata, Huyen Dinh, Masayuki Saimura, Arivazhagan Rajendran, Kazunari Matsuda, Takashi Morii

Abstract Recognition‐driven modification has been emerging as a novel approach to modifying biomolecular targets of interest site‐specifically and efficiently. To this end, protein modular adaptors (MAs) are the ideal reaction model for recognition‐driven modification of DNA as they consist of both a sequence‐specific DNA‐binding domain (DBD) and a self‐ligating protein‐tag. Coupling DNA recognition by DBD and the chemoselective reaction of the protein tag could provide a highly efficient...

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European Journal of Inorganic Chemistry

Halide Ion Migration and its Role at the Interfaces in Perovskite Solar Cells

Published: 23 November 2021

Author(s): Minjin Kim, Haeyeon Jun, Heejae Lee, Hindia Nahdi, Denis Tondelier, Yvan Bonnassieux, Jean‐Éric Bourée, Bernard Geffroy

Abstract Lead‐halide perovskite solar cells (PSCs) based on unusual semiconductors made with ions, have shown impressive improvement in photovoltaic performance in few years exceeding nowadays 25 % power conversion efficiency. However, PSCs suffer from a lack of stability and show significant hysteresis in current‐voltage curves, which are impeding commercialization. We confirmed the importance of halide ion migration in the hysteresis effect which has direct consequences on device efficiency....

thumbnail image: European Journal of Inorganic Chemistry

Chemistry - A European Journal

Dinuclear Zinc Catalyzed Enantioselective Dearomatization [3+2] Annulation of 2‐Nitrobenzofurans and 2‐Nitrobenzothiophenes

Published: 23 November 2021

Author(s): Peng Zhou, Yang Yi, Yuan‐Zhao Hua, Shi‐Kun Jia, Min‐Can Wang

Abstract The application of dinuclear zinc catalysts in a dearomatization reaction has been developed. Catalytic asymmetric dearomatization [3+2] annulations of 2‐nitrobenzofurans or 2‐nitrobenzothiophenes with CF3‐containing N‐unprotected isatin‐derived azomethine ylides catalyzed by dinuclear zinc catalysts are realized with excellent diastereomer ratios (dr) of 20 : 1 and enantiomeric excess (ee) of up to 99 %. This protocol provides a practical, straightforward access to structurally...

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European Journal of Inorganic Chemistry

An Unprecedented Cluster Unit in (BMIm)2[Hf9Cl14H8(AlCl4)6]

Published: 23 November 2021

Author(s): Jonas Jablonski, Jonas Bresien, Martin Köckerling

Abstract The reduction of HfCl4 with Li[AlH4] under ionothermal conditions using (BMIm)[AlCl4] as solvent and as reactant gives the compound (BMIm)2[Hf9Cl14H8(AlCl4)6] in moderate yield. It contains nona‐nuclear metalloid cluster units with an unprecedented arrangement of the metal atoms. This can be described by a polyhedron consisting of two trigonal bipyramids, which are fused in one basal Hf atom. The edges of the Hf9 polyhedron are bridged by Cl atoms and the apical sites Cl‐bonded to...

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Most-accessed articles from each Chemistry Europe, ACES, and GDCh journal

October 2021


Fang Zhang, Juewen Liu
Label-Free Colorimetric Biosensors Based on Aptamers and Gold Nanoparticles: A Critical Review [Review]
Anal. Sens. 2021, vol. 1, no. 1, p. 30

Rola Houhou, Thomas Bocklitz
Trends in artificial intelligence, machine learning, and chemometrics applied to chemical data [Review]
Anal. Sci. Adv. 2021, vol. 2, no. 3-4, p. 128

Alana Zülke, Yi Li, Peter Keil, Robert Burrell, Sacha Belaisch, Mangayarkarasi Nagarathinam, Michael P. Mercer, Harry E. Hoster
High-Energy Nickel-Cobalt-Aluminium Oxide (NCA) Cells on Idle: Anode- versus Cathode-Driven Side Reactions [Article]
Batteries Supercaps 2021, vol. 4, no. 6, p. 934

Hemanth Maddali, Catherine E. Miles, Joachim Kohn, Deirdre M. O'Carroll
Optical Biosensors for Virus Detection: Prospects for SARS-CoV-2/COVID-19 [Minireview]
ChemBioChem 2021, vol. 22, no. 7, p. 1176

Christian M. Heckmann, Francesca Paradisi
Looking Back: A Short History of the Discovery of Enzymes and How They Became Powerful Chemical Tools [Review]
ChemCatChem 2020, vol. 12, no. 24, p. 6082

Pooja Vadhva, Ji Hu, Michael J. Johnson, Richard Stocker, Michele Braglia, Dan J. L. Brett, Alexander J. E. Rettie
Electrochemical Impedance Spectroscopy for All-Solid-State Batteries: Theory, Methods and Future Outlook [Review]
ChemElectroChem 2021, vol. 8, no. 11, p. 1930

Keita Sakamoto, Akihiro Hakamata, Arihiro Iwasaki, Kiyotake Suenaga, Masashi Tsuda, Haruhiko Fuwa
Cover Feature: Total Synthesis, Stereochemical Revision, and Biological Assessment of Iriomoteolide-2a (Chem. Eur. J. 36/2019) [Cover Picture]
Chem. Eur. J. 2019, vol. 25, no. 36, p. 8429

Guilherme L. Tripodi, Max T. G. M. Derks, Floris P. J. T. Rutjes, Jana Roithová
Tracking Reaction Pathways by a Modular Flow Reactor Coupled to Electrospray Ionization Mass Spectrometry [Cover Profile]
Chemistry–Methods 2021, vol. 1, no. 10, p. 428

Zheng-Wang Qu, Hui Zhu, Sergey A. Katsyuba, Vera L. Mamedova, Vakhid A. Mamedov, Stefan Grimme
Acid-Catalyzed Rearrangements of 3-Aryloxirane-2-Carboxamides: Novel DFT Mechanistic Insights [Communication]
ChemistryOpen 2020, vol. 9, no. 7, p. 743

Miaofang Chi, Harry M. Meyer, Zili Wu, Liangbo Liang, Peter V. Bonnesen, Dale K. Hensley, Rui Peng, Yang Song, Cheng Ma, Bobby G. Sumpter, Adam J. Rondinone
High-Selectivity Electrochemical Conversion of CO2 to Ethanol using a Copper Nanoparticle/N-Doped Graphene Electrode [Full Paper]
ChemistrySelect 2016, vol. 1, no. 19, p. 6055

Antoine Daina, Vincent Zoete
A BOILED‐Egg To Predict Gastrointestinal Absorption and Brain Penetration of Small Molecules [Communication]
ChemMedChem 2016, vol. 11, no. 11, p. 1117

Thomas D. Svejstrup, Anamitra Chatterjee, Denis Schekin, Thomas Wagner, Julia Zach, Magnus J. Johansson, Giulia Bergonzini, Burkhard König
Effects of Light Intensity and Reaction Temperature on Photoreactions in Commercial Photoreactors [Communication]
ChemPhotoChem 2021, vol. 5, no. 9, p. 808

Thomas G. Mayerhöfer, Susanne Pahlow, Jürgen Popp
The Bouguer-Beer-Lambert Law: Shining Light on the Obscure [Review]
ChemPhysChem 2020, vol. 21, no. 18, p. 2029

Francesco Bisconti, Antonella Giuri, Gianluigi Marra, Alberto Savoini, Paolo Fumo, Rosamaria Marrazzo, Stefano Zanardi, Gianni Corso, Riccardo Po, Paolo Biagini, Eleonora Quadrivi, Riikka Suhonen, Thomas M. Kraft, Mari Ylikunnari, Andrea Listorti, Carola Esposito Corcione, Silvia Colella, Aurora Rizzo
Polymer-Assisted Single-Step Slot-Die Coating of Flexible Perovskite Solar Cells at Mild Temperature from Dimethyl Sulfoxide [Full Paper]
ChemPlusChem 2021, vol. 86, no. 10, p. 1442

Layla Filiciotto, Gadi Rothenberg
Biodegradable Plastics: Standards, Policies, and Impacts [Review]
ChemSusChem 2021, vol. 14, no. 1, p. 56

Anton I. Hanopolskyi, Viktoryia A. Smaliak, Alexander I. Novichkov, Sergey N. Semenov
Autocatalysis: Kinetics, Mechanisms and Design [Review]
ChemSystemsChem 2021, vol. 3, eLoc. e2000026

Saheed E. Elugoke, Abolanle S. Adekunle, Omolola E. Fayemi, Ekemini D. Akpan, Bhekie B. Mamba, El-Sayed M. Sherif, Eno E. Ebenso
Molecularly imprinted polymers (MIPs) based electrochemical sensors for the determination of catecholamine neurotransmitters - Review [REVIEW]
Electrochem. Sci. Adv. 2021, vol. 1, eLoc. e2000026

Mauricio Cattaneo, Giovanny A. Parada, Adam L. Tenderholt, Werner Kaminsky, James M. Mayer
Structural, Electronic, and Thermochemical Preference for Multi-PCET Reactivity of Ruthenium(II)-Amine and Ruthenium(IV)-Amido Complexes [Full Paper]
Eur. J. Inorg. Chem. 2021, p. 4066

Luca Capaldo, Davide Ravelli
Hydrogen Atom Transfer (HAT): A Versatile Strategy for Substrate Activation in Photocatalyzed Organic Synthesis [Microreview]
Eur. J. Org. Chem. 2017, p. 2056

Catharina Goedecke
Why Does Iodine Turn Starch Blue?
ChemistryViews 2016

Michael C. Willis, Edward J. Emmett
The Development and Application of Sulfur Dioxide Surrogates in Synthetic Organic Chemistry [Focus Review]
Asian J. Org. Chem. 2015, vol. 4, no. 7, p. 602

Stephanie C. C. van der Lubbe, Célia Fonseca Guerra
The Nature of Hydrogen Bonds: A Delineation of the Role of Different Energy Components on Hydrogen Bond Strengths and Lengths [Minireview]
Chem. Asian J. 2019, vol. 14, no. 16, p. 2760

B. Lilli Neumeier, Mikhail Khorenko, Frauke Alves, Oliver Goldmann, Joanna Napp, Ute Schepers, Holger M. Reichardt, Claus Feldmann
Fluorescent Inorganic-Organic Hybrid Nanoparticles [Focus Review]
ChemNanoMat 2019, vol. 5, no. 1, p. 24

Xiaoye Yu, Constantin G. Daniliuc, Fatmah Ali Alasmary, Armido Studer
Direct Access to α-Aminosilanes Enabled by Visible-Light-Mediated Multicomponent Radical Cross-Coupling [Research Article]
Angew. Chem. Int. Ed. 2021, vol. 60, no. 43, p. 23335

Abas Mohsenzadeh, Akram Zamani, Mohammad J. Taherzadeh
Bioethylene Production from Ethanol: A Review and Techno-economical Evaluation [Review]
ChemBioEng Rev. 2017, vol. 4, no. 2, p. 75

Özge Çepelioğullar Mutlu, Thomas Zeng
Challenges and Opportunities of Modeling Biomass Gasification in Aspen Plus: A  Review [Review]
Chem. Eng. Technol. 2020, vol. 43, no. 9, p. 1674

Nuria Sánchez-Bastardo, Robert Schlögl, Holger Ruland
Methane Pyrolysis for CO2-Free H2 Production: A Green Process to Overcome Renewable Energies Unsteadiness [Review]
Chem. Ing. Tech. 2020, vol. 92, no. 10, p. 1596

Manami Ishida, Dieter Weiß
Blausäure im Haushalt [Magazin]
Chem. Unserer Zeit 2021, vol. 55, no. 5, p. 359

Digitalisierung nach der Pandemie [Editorial]
CHEMKON 2021, vol. 28, no. 6, p. 234

Cover Picture Lebensmittelchemie 5/2021 [Cover Picture]
Lebensmittelchemie 2021, vol. 75, no. 5

Sonja Herres-Pawlis, Johannes Liermann
Den Datenschatz endlich heben [Leitartikel]
Nachr. Chem. 2021, vol. 69, no. 10, p. 3

Most cited articles from Chemistry Europe, ACES, and GDCh journals

Articles on this list are the most frequently cited ones among those published in 2018 or 2019 according to Web of Science. They have contributed the most to the journal's impact factor in 2020.


Jing Pan, Xin Long Tian, Shahid Zaman, Zehua Dong, Hongfang Liu, Ho Seok Park, Bao Yu Xia
Recent Progress on Transition Metal Oxides as Bifunctional Catalysts for Lithium-Air and Zinc-Air Batteries [Minireview]
Batteries Supercaps 2019, vol. 2, pp. 336–347

Veeresh Juturu, Jin Chuan Wu
Heterologous Protein Expression in Pichia pastoris: Latest Research Progress and Applications [Review]
ChemBioChem 2018, vol. 19, pp. 7–21

Tingmin Di, Quanlong Xu, WingKei Ho, Hua Tang, Quanjun Xiang, Jiaguo Yu
Review on Metal Sulphide-based Z-scheme Photocatalysts [Review]
ChemCatChem 2019, vol. 11, pp. 1394–1411

Lantao Liu, Yanli Zhou, Shuang Liu, Maotian Xu
The Applications of Metal−Organic Frameworks in Electrochemical Sensors [Review]
ChemElectroChem 2018, vol. 5, pp. 6–19

Min Feng, Ming-Liang Tong
Single Ion Magnets from 3d to 5f: Developments and Strategies [Minireview]
Chem. Eur. J. 2018, vol. 24, pp. 7574–7594

Massimo Baroncini, Lorenzo Casimiro, Christiaan de Vet, Jessica Groppi, Serena Silvi, Alberto Credi
Making and Operating Molecular Machines: A Multidisciplinary Challenge [Minireview]
ChemistryOpen 2018, vol. 7, pp. 169–179

Patil S. Basavarajappa, Bhojya Naik H. Seethya, Nagaraju Ganganagappa, Kumaraswamy B. Eshwaraswamy, Raghava Reddy Kakarla
Enhanced Photocatalytic Activity and Biosensing of Gadolinium Substituted BiFeO3 Nanoparticles [Full Paper]
ChemistrySelect 2018, vol. 3, pp. 9025–9033

Deepti Goyal, Amandeep Kaur, Bhupesh Goyal
Benzofuran and Indole: Promising Scaffolds for Drug Development in Alzheimer's Disease [Review]
ChemMedChem 2018, vol. 13, pp. 1275–1299

Hiroki Tanaka, Yoshihisa Inoue, Tadashi Mori
Circularly Polarized Luminescence and Circular Dichroisms in Small Organic Molecules: Correlation between Excitation and Emission Dissymmetry Factors [Review]
ChemPhotoChem 2018, vol. 2, pp. 386–402

Weiyin Gao, Chenxin Ran, Jun Xi, Bo Jiao, Wenwen Zhang, Mincai Wu, Xun Hou, Zhaoxin Wu
High-Quality Cs2AgBiBr6 Double Perovskite Film for Lead-Free Inverted Planar Heterojunction Solar Cells with 2.2 % Efficiency [Communication]
ChemPhysChem 2018, vol. 19, pp. 1696–1700

Achini Japahuge, Tao Zeng
Theoretical Studies of Singlet Fission: Searching for Materials and Exploring Mechanisms [Review]
ChemPlusChem 2018, vol. 83, pp. 146–182

Peixun Xiong, Xinxin Zhao, Yunhua Xu
Nitrogen-Doped Carbon Nanotubes Derived from Metal-Organic Frameworks for Potassium-Ion Battery Anodes [Full Paper]
ChemSusChem 2018, vol. 11, pp. 202–208

Nadja Stucke, Benedikt M. Flöser, Thomas Weyrich, Felix Tuczek
Nitrogen Fixation Catalyzed by Transition Metal Complexes: Recent Developments [Microreview]
Eur. J. Inorg. Chem. 2018, pp. 1337–1355

Davin Tan, Tomislav Friščić
Mechanochemistry for Organic Chemists: An Update [Microreview]
Eur. J. Org. Chem. 2018, pp. 18–33

Esther von Grotthuss, Alexandra John, Thomas Kaese, Matthias Wagner
Doping Polycyclic Aromatics with Boron for Superior Performance in Materials Science and Catalysis [Focus Review]
Asian J. Org. Chem. 2018, vol. 7, pp. 37–53

Min-Hua Huang, Wen-Juan Hao, Bo Jiang
Recent Advances in Radical-Enabled Bicyclization and Annulation/1,n-Bifunctionalization Reactions [Focus Review]
Chem. Asian J. 2018, vol. 13, pp. 2958–2977

Amit Kumar, Qiang Xu
Two-Dimensional Layered Materials as Catalyst Supports [Focus Review]
ChemNanoMat 2018, vol. 4, pp. 28–40

Leyre Marzo, Santosh K. Pagire, Oliver Reiser, Burkhard König
Visible-Light Photocatalysis: Does It Make a Difference in Organic Synthesis? [Review]
Angew. Chem. Int. Ed. 2018, vol. 57, pp. 10034–10072

Sayantani Sikdar, Madhusree Kundu
A Review on Detection and Abatement of Heavy Metals [Review]
ChemBioEng Rev. 2018, vol. 5, pp. 18–29

Marwa Elkady, Hassan Shokry, Hesham Hamad
Microwave-Assisted Synthesis of Magnetic Hydroxyapatite for Removal of Heavy Metals from Groundwater [Research Article]
Chem. Eng. Technol. 2018, vol. 41, pp. 553–562

Jaqueline Daniel-Gromke, Nadja Rensberg, Velina Denysenko, Walter Stinner, Tina Schmalfuß, Mattes Scheftelowitz, Michael Nelles, Jan Liebetrau
Current Developments in Production and Utilization of Biogas and Biomethane in Germany [Review]
Chem. Ing. Tech. 2018, vol. 90, pp. 17–35

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Magazine of Chemistry Europe (16 European Chemical Societies) published by Wiley-VCH