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Chemistry - A European Journal

Efficient Synthesis of a NHC‐Coordinated Trisilacyclopropylidene and Its Coordination Behavior

Published: 22 June 2018

Author(s): Benedikt J. Guddorf, Alexander Hepp, Felicitas Lips

Abstract With a co‐reduction procedure using 2 equivalents Mes2SiCl2 and 1 equivalent NHCiPr2Me2→SiCl4 an NHC‐adduct of a trisilacyclopropylidene (SiMes2)2SiNHCiPr2Me2 1 was synthesized. Addition of NHCMe4 to 1 results in quantitative carbene exchange under release of NHCiPr2Me2 to yield (SiMes2)2SiNHCMe4 2. Both NHC‐coordinated trisilacyclopropylidenes coordinate to BH3. In reaction of 1 with SiMe3N3 a NHC‐coordinated trisilane with an exocyclic Si=N double bond is...

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ChemSusChem

Charge and Potential Balancing for Optimized Capacitive Deionization Using Lignin‐Derived, Low‐Cost Activated Carbon Electrodes

Published: 22 June 2018

Author(s): Rafael Linzmeyer Zornitta, Pattarachai Srimuk, Juhan Lee, Benjamin Krüner, Mesut Aslan, Luis Augusto Martins Ruotolo, Volker Presser

Abstract Lignin‐derived carbon is introduced as a promising electrode material for water desalination by using capacitive deionization (CDI). Lignin is a low‐cost precursor that is obtained from the cellulose and ethanol industries, and we used carbonization and subsequent KOH activation to obtain highly porous carbon. CDI cells with a pair of lignin‐derived carbon electrodes presented an initially high salt adsorption capacity but...

ChemSusChem

Pyrosynthesis of Na ₃ V ₂ (PO ₄ ) ₃ @C Cathodes for Safe and Low‐Cost Aqueous Hybrid Batteries

Published: 22 June 2018

Author(s): Saiful Islam, Muhammad Hilmy Alfaruqi, Dimas Yunianto Putro, Vinod Mathew, Sungjin Kim, Jeonggeun Jo, Seokhun Kim, Yang‐Kook Sun, Kwangho Kim, Jaekook Kim

Abstract Rechargeable hybrid aqueous batteries (ReHABs) have emerged as promising sustainable energy‐storage devices because all components are environmentally benign and abundant. In this study, a carbon‐wrapped sponge‐like Na3V2(PO4)3 nanoparticle (NVP@C) cathode is prepared by a simple pyrosynthesis for use in the ReHAB system with impressive rate capability and high cyclability. A high‐resolution X‐ray diffraction study confirmed the...

ChemPhysChem

Non‐steric Interactions Predict the Trend and Steric Interactions the Offset of Protein Stability in Cells

Published: 22 June 2018

Author(s): Caitlin M. Davis, Martin Gruebele

Abstract Although biomolecules evolved to function in the cell, most biochemical assays are carried out in vitro. In‐cell studies highlight how steric and non‐steric interactions modulate protein folding and interactions. VlsE and PGK present two extremes of chemical behavior in the cell: the extracellular protein VlsE is destabilized in eukaryotic cells, whereas the cytoplasmic protein PGK is stabilized. VlsE and PGK are benchmarks in a...

ChemPhysChem

Modeling Quantum Kinetics in Ion Traps: State‐changing Collisions for OH ⁺ ( $^{3} Σ^{-}$ ) Ions with He as a Buffer Gas

Published: 22 June 2018

Author(s): L. González‐Sánchez, R. Wester, F.A. Gianturco

Abstract We present quantum scattering calculations for rotational state‐changing cross sections and rates, up to about 50 K of ion translational temperatures, for the OH+ molecular ion in collision with He atoms as the buffer gas in the trap. The results are obtained both by using the correct spin‐rotation coupling of angular momenta and also within a recoupling scheme that treats the molecular target as a pseudo‐( ...

ChemPhysChem

Mesoporous ZnFe ₂ O ₄ Photoanodes with Template‐tailored Mesopores and Temperature‐dependent Photocurrents

Published: 22 June 2018

Author(s): Kristin Kirchberg, Songcan Wang, Lianzhou Wang, Roland Marschall

Abstract Mesoporous ZnFe2O4 photoanodes have been prepared via dip‐coating utilizing the evaporation‐induced self‐assembly of two different block‐copolymer templates to investigate the influence of pore geometry on the photoelectrochemcial performance of those earth‐abundant photoelectrodes. The use of commercial block copolymers, triblock copolymer Pluronic® F127 and the diblock copolymer PIB3000 as templates, leads to different pore...

European Journal of Inorganic Chemistry

Fluorescent Dyes in Organometallic Chemistry: Coumarin‐Tagged NHC–Metal Complexes

Published: 22 June 2018

Author(s): Oliver Halter, Herbert Plenio

7‐NEt2‐ and julolidene‐coumarin‐substituted azolium salts were synthesized and used to prepare the respective coumarin‐substituted NHC–metal complexes: [AuCl(NHC)], [PdCl(allyl)(NHC)], [MCl(CO)2(NHC)] (M = Rh, Ir), [MCl(cod)(NHC)] (M = Rh, Ir), [PdCl2(Cl‐py)(NHC)], [PdC(allyl)]2, and [RuCl2(ind)(NHC)(SIMes)] – sorted according to the respective fluorescence quantum yields of between φ = 0.70 [Au] and φ = 0.005 [Ru]. The fluorescence intensity of the complexes...

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Chemistry - A European Journal

Photogeneration of Microporous Amorphous Coordination Polymers from Organometallic Ionic Liquids

Published: 21 June 2018

Author(s): Takahiro Ueda, Takumi Tominaga, Tomoyuki Mochida, Kazuyuki Takahashi, Seiji Kimura

Abstract Ruthenium‐containing organometallic ionic liquids with the B(CN)4 anion were developed that generate microporous amorphous coordination polymers upon UV irradiation. UV light irradiation of [Ru(C5H5)(C6H5R)][B(CN)4] (R=butyl, ethyl, octyl) quantitatively generated a yellow powder of a coordination polymer with the formula [Ru(C5H5){B(CN)4}]n. In this reaction, the arene ligand is eliminated by UV irradiation and coordination polymer is formed by...

Chemistry - A European Journal

A Trichromatic and White‐Light‐Emitting MOF Composite for Multi‐Dimensional and Multi‐Response Ratiometric Luminescent Sensing

Published: 21 June 2018

Author(s): Yue Dai, Jian‐Jun Zhang, Shu‐Qin Liu, Huajun Zhou, Ying‐Ji Sun, Yu‐Zhen Pan, Jun Ni, Jing‐Si Yang

Abstract Present here is a new dual ratiometric luminescent probe D which is a trichromatic and white‐light‐emitting metal‐organic framework (MOF) composite facilely obtained by incorporating red/green‐emitting complex modules into a blue‐emitting MOF. Probe D exhibits remarkable capabilities of sensing different volatile organic solvents (VOSs) via 2D code recognition of the two VOS‐dependent MOF ligand‐to‐module ratios of the emission‐peak...

Chemistry - A European Journal

Uncommon Optical Properties and Silver‐Responsive Turn‐Off/On Luminescence in a Pt ^II Heteroleptic Dithiolene Complex

Published: 21 June 2018

Author(s): Salahuddin S. Attar, Flavia Artizzu, Luciano Marchiò, Davide Espa, Luca Pilia, Maria F. Casula, Angela Serpe, Maddalena Pizzotti, Alessio Orbelli‐Biroli, Paola Deplano

Abstract Complex [Pt(iPr2pipdt)(Quinoxdt)] (iPr2pipdt=1,4‐diisopropyl‐piperazine‐2,3‐dithione; Quinoxdt=[1,4]dithiino[2,3‐b]quinoxaline‐2,3‐dithiolate) exhibits a remarkable green emission at 570 nm (room temperature), which is above the lowest excited state. The complex is characterized by negative solvatochromism as well as a high second‐order polarizability. Addition of AgI ions induces 1) hypsochromic shift of the lowest frequencies and...

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Most-accessed articles from each ChemPubSoc Europe, ACES, and GDCh journal

March 2018


	Zhang Luo, Bing Liu Shape-Tunable Colloids from Structured Liquid Droplet Templates [Cover Picture] Angew. Chem. Int. Ed. 10.1002/anie.201802726

	Coline Jumeaux, Olov Wahlsten, Stephan Block, Eunjung Kim, Rona Chandrawati, Philip D. Howes, Fredrik Höök, Molly M. Stevens MicroRNA Detection by DNA-Mediated Liposome Fusion [Communication] ChemBioChem 2018, vol. 19, p. 434

	Isabela C. Man, Hai-Yan Su, Federico Calle-Vallejo, Heine A. Hansen, José I. Martínez, Nilay G. Inoglu, John Kitchin, Thomas F. Jaramillo, Jens K. Nørskov, Jan Rossmeisl Universality in Oxygen Evolution Electrocatalysis on Oxide Surfaces [Full Paper] ChemCatChem 2011, vol. 3, p. 1159

	Matthias Schäfer, Bernhard Hauck, Jochen Kuhn, Roland Ulber Analytik mit Licht - Das Smartphone-Photometer [Artikel] Chem. Unserer Zeit 2018, vol. 52, p. 52

	Balaram Mukhopadhyay, Rituparna Das Chemical O-Glycosylations: An Overview [Review] ChemistryOpen 2016, vol. 5, p. 401

	Hanshen Xin, Xike Gao Application of Azulene in Constructing Organic Optoelectronic Materials: New Tricks for an Old Dog [Minireview] ChemPlusChem 2017, vol. 82, p. 945

	Miaofang Chi, Harry M. Meyer, Zili Wu, Liangbo Liang, Peter V. Bonnesen, Dale K. Hensley, Rui Peng, Yang Song, Cheng Ma, Bobby G. Sumpter, Adam J. Rondinone High-Selectivity Electrochemical Conversion of CO₂ to Ethanol using a Copper Nanoparticle/N-Doped Graphene Electrode [Full Paper] ChemistrySelect 2016, vol. 1, p. 6055

	Hubert Rauscher, Kirsten Rasmussen, Birgit Sokull-Klüttgen Regulatory Aspects of Nanomaterials in the EU [Research Article] Chem. Ing. Tech. 2017, vol. 89, p. 224

	Abas Mohsenzadeh, Akram Zamani, Mohammad J. Taherzadeh Bioethylene Production from Ethanol: A Review and Techno-economical Evaluation [Review] ChemBioEng Rev. 2017, vol. 4, p. 75

	Robert A. W. Dryfe, Briony Setterfield-Price, Joanne Tory, František Hartl [M(CO)₄(2,2'-bipyridine)] (M=Cr, Mo, W) Complexes as Efficient Catalysts for Electrochemical Reduction of CO₂ at a Gold Electrode [Communication] ChemElectroChem 2015, vol. 2, p. 213

	Yinghui Xue, Qin Zhang, Tao Zhang, Lei Fu Black Phosphorus: Properties, Synthesis, and Applications in Energy Conversion and Storage [Focus Review] ChemNanoMat 2017, vol. 3, p. 352

	Maximilian Koy, Frederik Sandfort, Adrian Tlahuext-Aca, Linda Quach, Constantin G. Daniliuc, Frank Glorius Palladium-Catalyzed Decarboxylative Heck-Type Coupling of Activated Aliphatic Carboxylic Acids Enabled by Visible Light [Communication] Chem. Eur. J. 2018, vol. 24, p. 4552

	Jian Lv, Qi Zhang, Mao Cai, Yanfang Han, Sanzhong Luo Aromatic Aminocatalysis [Focus Review] Chem. Asian J. 2018, vol. 13, p. 740

	Hidetoshi Noda, Naoya Kumagai, Masakatsu Shibasaki Abstract [Focus Review] Asian J. Org. Chem. 10.1002/ajoc.201800013

	Albert J. Kooistra, Márton Vass, Ross McGuire, Rob Leurs, Iwan J. P. de Esch, Gert Vriend, Stefan Verhoeven, Chris de Graaf 3D-e-Chem: Structural Cheminformatics Workflows for Computer-Aided Drug Discovery [Full Paper] ChemMedChem 2018, vol. 13, p. 614

	Zhoufeng Bian, Sonali Das, Ming Hui Wai, Plaifa Hongmanorom, Sibudjing Kawi A Review on Bimetallic Nickel-Based Catalysts for CO₂ Reforming of Methane [Review] ChemPhysChem 2017, vol. 18, p. 3117

	Turkan Gamze Ulusoy Ghobadi, Amir Ghobadi, Ekmel Ozbay, Ferdi Karadas Strategies for Plasmonic Hot-Electron-Driven Photoelectrochemical Water Splitting [Review] ChemPhotoChem 2018, vol. 2, p. 161

	An-Na Cho, Nam-Gyu Park Impact of Interfacial Layers in Perovskite Solar Cells [Review] ChemSusChem 2017, vol. 10, p. 3687

	Jeffrey A. Rood, Sondra E. Hinman, Bruce C. Noll, Kenneth W. Henderson The Use of Halide-Substituted Anilines for the Formation of Magnesium Imides [Full Paper] Eur. J. Inorg. Chem. 2008, p. 3935

	D. B. Ramachary [Author Profile] Eur. J. Org. Chem. 10.1002/ejoc.201800182

	46. Deutscher Lebensmittelchemikertag 2017 in Würzburg [Tagung] Lebensmittelchemie 2018, vol. 72, p. 1

	Peter Chen Chemistry 4.0 [Leitartikel] Nachr. Chem. 2018, vol. 66, p. 203

	Ira Caspari, Gisela Weber-Peukert, Nicole Graulich Der Einsatz von Modellen zum Erkenntnisgewinn / Eine Unterrichtseinheit zur Förderung der Modellkompetenz im Kontext „Batterie“ unter explizitem Einbezug von Schülervorstellungen [Aus der Schule] CHEMKON 2018, vol. 25, p. 23

	Catharina Goedecke Why Does Iodine Turn Starch Blue? ChemViews Magazine 2016

Most cited articles from each ChemPubSoc Europe, ACES, and GDCh journal

2016


	Shoujun Zhu, Qingnan Meng, Lei Wang, Junhu Zhang, Yubin Song, Han Jin, Kai Zhang, Hongchen Sun, Haiyu Wang, Bai Yang Highly Photoluminescent Carbon Dots for Multicolor Patterning, Sensors, and Bioimaging Angew. Chem. Int. Ed. 2013, vol. 52, pp. 3953–3957

	Balayeshwanth R. Vummidi, Jawad Alzeer, Nathan W. Luedtke Fluorescent Probes for G-Quadruplex Structures [Review] ChemBioChem 2013, vol. 14, pp. 540–558

	Zhi-Yuan Gu, Jihye Park, Aaron Raiff, Zhangwen Wei, Hong-Cai Zhou Metal–Organic Frameworks as Biomimetic Catalysts [Minireview] ChemCatChem 2014, vol. 6, pp. 67–75

	Anthony J. Arduengo, Roland Krafczyk Auf der Suche nach Stabilen Carbenen [Organische Chemie] Chem. Unserer Zeit 1998, vol. 32, pp. 6–14

	Marc Steinmetz, Stefan Grimme Benchmark Study of the Performance of Density Functional Theory for Bond Activations with (Ni,Pd)-Based Transition-Metal Catalysts [Full Paper] ChemistryOpen 2013, vol. 2, pp. 115–124

	Philipp Scharf, Jens Müller Nucleic Acids With Metal-Mediated Base Pairs and Their Applications [Review] ChemPlusChem 2013, vol. 78, pp. 20–34

	Philipp Kaiser, Rajabhau?Bajirao Unde, Christoph Kern, Andreas Jess Production of Liquid Hydrocarbons with CO₂ as Carbon Source based on Reverse Water-Gas Shift and Fischer-Tropsch Synthesis [Research Article] Chem. Ing. Tech. 2013, vol. 85, pp. 489–499

	Xiaosi Zhou, Yu-Guo Guo Highly Disordered Carbon as a Superior Anode Material for Room-Temperature Sodium-Ion Batteries [Communication] ChemElectroChem 2014, vol. 1, pp. 83–86

	Chuanxi Wang, Zhenzhu Xu, Chi Zhang Polyethyleneimine-Functionalized Fluorescent Carbon Dots: Water Stability, pH Sensing, and Cellular Imaging [Full Paper] ChemNanoMat 2015, vol. 1, pp. 122–127

	Konggang Qu, Jiasi Wang, Jinsong Ren, Xiaogang Qu Carbon Dots Prepared by Hydrothermal Treatment of Dopamine as an Effective Fluorescent Sensing Platform for the Label-Free Detection of Iron(III) Ions and Dopamine [Full Paper] Chem. Eur. J. 2013, vol. 19, pp. 7243–7249

	Yinuo Wu, Jun Wang, Fei Mao, Fuk Yee Kwong Palladium-Catalyzed Cross-Dehydrogenative Functionalization of C(sp²)–H Bonds [Focus Review] Chem. Asian J. 2014, vol. 9, pp. 26–47

	Naohiko Yoshikai, Ye Wei Synthesis of Pyrroles, Indoles, and Carbazoles through Transition-Metal-Catalyzed C–H Functionalization [Review] Asian J. Org. Chem. 2013, vol. 2, pp. 466–478

	Lluís Ballell, Robert H. Bates, Rob J. Young, Daniel Alvarez-Gomez, Emilio Alvarez-Ruiz, Vanessa Barroso, Delia Blanco, Benigno Crespo, Jaime Escribano, Rubén González, Sonia Lozano, Sophie Huss, Angel Santos-Villarejo, José Julio Martín-Plaza, Alfonso Mendoza, María José Rebollo-Lopez, Modesto Remuiñan-Blanco, José Luis Lavandera, Esther Pérez-Herran, Francisco Javier Gamo-Benito, José Francisco García-Bustos, David Barros, Julia P. Castro, Nicholas Cammack Fueling Open-Source Drug Discovery: 177 Small-Molecule Leads against Tuberculosis [Full Paper] ChemMedChem 2013, vol. 8, pp. 313–321

	Peter Politzer, Jane S. Murray Halogen Bonding: An Interim Discussion [Review] ChemPhysChem 2013, vol. 14, pp. 278–294

	Volker Hessel, Dana Kralisch, Norbert Kockmann, Timothy Noël, Qi Wang Novel Process Windows for Enabling, Accelerating, and Uplifting Flow Chemistry [Review] ChemSusChem 2013, vol. 6, pp. 746–789

	Helena J. Shepherd, Gábor Molnár, William Nicolazzi, Lionel Salmon, Azzedine Bousseksou Spin Crossover at the Nanometre Scale [Microreview] Eur. J. Inorg. Chem. 2013, pp. 653–661

	Junichiro Yamaguchi, Kei Muto, Kenichiro Itami Recent Progress in Nickel-Catalyzed Biaryl Coupling [Microreview] Eur. J. Org. Chem. 2013, pp. 19–30

	David Schweinfurth, Naina Deibel, Fritz Weisser, Biprajit Sarkar Mit Klick zu neuen Liganden [Magazin] Nachr. Chem. 2011, vol. 59, pp. 937–941