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Chemistry - A European Journal

Hypophosphites as Eco‐Compatible Fuels for Membrane‐Free Direct Liquid Fuel Cells

Published: 22 June 2018

Author(s): Renhe Wang, Mengjia Wu, Servane Haller, Pascal Métivier, Yonggang Wang, Yongyao Xia

Abstract Crossover of liquid fuel remains a severe problem for conventional direct liquid fuel cells even when polymer electrolyte membranes are applied. Herein, we report for the first time a membrane‐free direct liquid fuel cell powered by alkaline hypophosphite solution. The proof‐of‐concept fuel cell yields a peak power density of 32 mW cm−2 under air flow at room temperature. The removal of the polymer electrolyte membrane is attributed to...

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Chemistry - A European Journal

Spiro‐epoxyglycosides as Activity‐Based Probes for Glycoside Hydrolase Family 99 Endomannosidase/Endomannanase

Published: 22 June 2018

Author(s): Sybrin P. Schröder, Wouter W. Kallemeijn, Marjoke F. Debets, Thomas Hansen, Lukasz F. Sobala, Zalihe Hakki, Spencer J. Williams, Thomas J. M. Beenakker, Johannes M. F. G. Aerts, Gijsbert A. van der Marel, Jeroen D. C. Codée, Gideon J. Davies, Herman S. Overkleeft

Abstract N‐Glycans direct protein function, stability, folding and targeting, and influence immunogenicity. While most glycosidases that process N‐glycans cleave a single sugar residue at a time, enzymes from glycoside hydrolase family 99 are endo‐acting enzymes that cleave within complex N‐glycans. Eukaryotic Golgi endo‐1,2‐α‐mannosidase cleaves glucose‐substituted mannose within immature glucosylated high‐mannose N‐glycans in the secretory ...

thumbnail image: Chemistry - A European Journal

Chemistry - A European Journal

Gold(I) Complexes Containing Phosphanyl‐ and Arsanylborane Ligands

Published: 22 June 2018

Author(s): Jens Braese, Alexander Schinabeck, Michael Bodensteiner, Hartmut Yersin, Alexey Y. Timoshkin, Manfred Scheer

Abstract The structural and photophysical properties of a series of new AuI compounds have been studied. The reactions of AuCl(tht) with the phosphanyl‐ and arsanylboranes RR′EBH2NMe3 (E=P, As; R=H, Ph; R′=H, Ph, tBu) afford the complexes [AuCl(RR′EBH2NMe3)]. In the solid state, [AuCl(H2PBH2NMe3)]2 (2 a) is a dimer showing unsupported intermolecular aurophilic interactions with short Au⋅⋅⋅Au distances. In contrast, [AuCl(H2AsBH2NMe3)]n (2 b) aggregates to form 1D...

thumbnail image: Chemistry - A European Journal

Chemistry - A European Journal

MultiValent Group 14 Chalcogenide Architectures from Ionic Liquids 0DCsSn II 4 Ge IV 4 Se 10 4 7 and 2DSn II Ge IV 4 Se 10 2

Published: 22 June 2018

Author(s): Silke Santner, Alexander Wolff, Michael Ruck, Stefanie Dehnen

Abstract In order to explore if and how salts comprising polycations and salts comprising polyanions might interact, the [AlBr4]− salt of the [Pt@Bi10]4+ cluster cation was added to the reaction mixture for the synthesis of the supersphere cluster anion [Ge24Sn36Se132]24− from Cs4[Ge4Se10]⋅H2O and SnCl4⋅5 H2O under ionothermal conditions at 120 °C. Indeed, the reaction yields two new compounds, depending on the cation of the used ionic liquid. Apparently,...

thumbnail image: Chemistry - A European Journal

Chemistry - A European Journal

Efficient Synthesis of a NHC‐Coordinated Trisilacyclopropylidene and Its Coordination Behavior

Published: 22 June 2018

Author(s): Benedikt J. Guddorf, Alexander Hepp, Felicitas Lips

Abstract With a co‐reduction procedure using 2 equivalents Mes2SiCl2 and 1 equivalent NHCiPr2Me2→SiCl4 an NHC‐adduct of a trisilacyclopropylidene (SiMes2)2SiNHCiPr2Me2 1 was synthesized. Addition of NHCMe4 to 1 results in quantitative carbene exchange under release of NHCiPr2Me2 to yield (SiMes2)2SiNHCMe4 2. Both NHC‐coordinated trisilacyclopropylidenes coordinate to BH3. In reaction of 1 with SiMe3N3 a NHC‐coordinated trisilane with an exocyclic Si=N double bond is...

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ChemSusChem

Charge and Potential Balancing for Optimized Capacitive Deionization Using Lignin‐Derived, Low‐Cost Activated Carbon Electrodes

Published: 22 June 2018

Author(s): Rafael Linzmeyer Zornitta, Pattarachai Srimuk, Juhan Lee, Benjamin Krüner, Mesut Aslan, Luis Augusto Martins Ruotolo, Volker Presser

Abstract Lignin‐derived carbon is introduced as a promising electrode material for water desalination by using capacitive deionization (CDI). Lignin is a low‐cost precursor that is obtained from the cellulose and ethanol industries, and we used carbonization and subsequent KOH activation to obtain highly porous carbon. CDI cells with a pair of lignin‐derived carbon electrodes presented an initially high salt adsorption capacity but...

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ChemSusChem

Pyrosynthesis of Na 3 V 2 (PO 4 ) 3 @C Cathodes for Safe and Low‐Cost Aqueous Hybrid Batteries

Published: 22 June 2018

Author(s): Saiful Islam, Muhammad Hilmy Alfaruqi, Dimas Yunianto Putro, Vinod Mathew, Sungjin Kim, Jeonggeun Jo, Seokhun Kim, Yang‐Kook Sun, Kwangho Kim, Jaekook Kim

Abstract Rechargeable hybrid aqueous batteries (ReHABs) have emerged as promising sustainable energy‐storage devices because all components are environmentally benign and abundant. In this study, a carbon‐wrapped sponge‐like Na3V2(PO4)3 nanoparticle (NVP@C) cathode is prepared by a simple pyrosynthesis for use in the ReHAB system with impressive rate capability and high cyclability. A high‐resolution X‐ray diffraction study confirmed the...

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ChemPhysChem

Non‐steric Interactions Predict the Trend and Steric Interactions the Offset of Protein Stability in Cells

Published: 22 June 2018

Author(s): Caitlin M. Davis, Martin Gruebele

Abstract Although biomolecules evolved to function in the cell, most biochemical assays are carried out in vitro. In‐cell studies highlight how steric and non‐steric interactions modulate protein folding and interactions. VlsE and PGK present two extremes of chemical behavior in the cell: the extracellular protein VlsE is destabilized in eukaryotic cells, whereas the cytoplasmic protein PGK is stabilized. VlsE and PGK are benchmarks in a...

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ChemPhysChem

Modeling Quantum Kinetics in Ion Traps: State‐changing Collisions for OH + ( 3Σ- ) Ions with He as a Buffer Gas

Published: 22 June 2018

Author(s): L. González‐Sánchez, R. Wester, F.A. Gianturco

Abstract We present quantum scattering calculations for rotational state‐changing cross sections and rates, up to about 50 K of ion translational temperatures, for the OH+ molecular ion in collision with He atoms as the buffer gas in the trap. The results are obtained both by using the correct spin‐rotation coupling of angular momenta and also within a recoupling scheme that treats the molecular target as a pseudo‐( ...

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ChemPhysChem

Mesoporous ZnFe 2 O 4 Photoanodes with Template‐tailored Mesopores and Temperature‐dependent Photocurrents

Published: 22 June 2018

Author(s): Kristin Kirchberg, Songcan Wang, Lianzhou Wang, Roland Marschall

Abstract Mesoporous ZnFe2O4 photoanodes have been prepared via dip‐coating utilizing the evaporation‐induced self‐assembly of two different block‐copolymer templates to investigate the influence of pore geometry on the photoelectrochemcial performance of those earth‐abundant photoelectrodes. The use of commercial block copolymers, triblock copolymer Pluronic® F127 and the diblock copolymer PIB3000 as templates, leads to different pore...

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Most-accessed articles from each ChemPubSoc Europe, ACES, and GDCh journal

March 2018

 


Zhang Luo, Bing Liu
Shape-Tunable Colloids from Structured Liquid Droplet Templates [Cover Picture]
Angew. Chem. Int. Ed. 10.1002/anie.201802726

Coline Jumeaux, Olov Wahlsten, Stephan Block, Eunjung Kim, Rona Chandrawati, Philip D. Howes, Fredrik Höök, Molly M. Stevens
MicroRNA Detection by DNA-Mediated Liposome Fusion [Communication]
ChemBioChem 2018, vol. 19, p. 434

Isabela C. Man, Hai-Yan Su, Federico Calle-Vallejo, Heine A. Hansen, José I. Martínez, Nilay G. Inoglu, John Kitchin, Thomas F. Jaramillo, Jens K. Nørskov, Jan Rossmeisl
Universality in Oxygen Evolution Electrocatalysis on Oxide Surfaces [Full Paper]
ChemCatChem 2011, vol. 3, p. 1159

Matthias Schäfer, Bernhard Hauck, Jochen Kuhn, Roland Ulber
Analytik mit Licht - Das Smartphone-Photometer [Artikel]
Chem. Unserer Zeit 2018, vol. 52, p. 52

Balaram Mukhopadhyay, Rituparna Das
Chemical O-Glycosylations: An Overview [Review]
ChemistryOpen 2016, vol. 5, p. 401

Hanshen Xin, Xike Gao
Application of Azulene in Constructing Organic Optoelectronic Materials: New Tricks for an Old Dog [Minireview]
ChemPlusChem 2017, vol. 82, p. 945

Miaofang Chi, Harry M. Meyer, Zili Wu, Liangbo Liang, Peter V. Bonnesen, Dale K. Hensley, Rui Peng, Yang Song, Cheng Ma, Bobby G. Sumpter, Adam J. Rondinone
High-Selectivity Electrochemical Conversion of CO2 to Ethanol using a Copper Nanoparticle/N-Doped Graphene Electrode [Full Paper]
ChemistrySelect 2016, vol. 1, p. 6055

Hubert Rauscher, Kirsten Rasmussen, Birgit Sokull-Klüttgen
Regulatory Aspects of Nanomaterials in the EU [Research Article]
Chem. Ing. Tech. 2017, vol. 89, p. 224

Abas Mohsenzadeh, Akram Zamani, Mohammad J. Taherzadeh
Bioethylene Production from Ethanol: A Review and Techno-economical Evaluation [Review]
ChemBioEng Rev. 2017, vol. 4, p. 75

Robert A. W. Dryfe, Briony Setterfield-Price, Joanne Tory, František Hartl
[M(CO)4(2,2'-bipyridine)] (M=Cr, Mo, W) Complexes as Efficient Catalysts for Electrochemical Reduction of CO2 at a Gold Electrode [Communication]
ChemElectroChem 2015, vol. 2, p. 213

Yinghui Xue, Qin Zhang, Tao Zhang, Lei Fu
Black Phosphorus: Properties, Synthesis, and Applications in Energy Conversion and Storage [Focus Review]
ChemNanoMat 2017, vol. 3, p. 352

Maximilian Koy, Frederik Sandfort, Adrian Tlahuext-Aca, Linda Quach, Constantin G. Daniliuc, Frank Glorius
Palladium-Catalyzed Decarboxylative Heck-Type Coupling of Activated Aliphatic Carboxylic Acids Enabled by Visible Light [Communication]
Chem. Eur. J. 2018, vol. 24, p. 4552

Jian Lv, Qi Zhang, Mao Cai, Yanfang Han, Sanzhong Luo
Aromatic Aminocatalysis [Focus Review]
Chem. Asian J. 2018, vol. 13, p. 740

Hidetoshi Noda, Naoya Kumagai, Masakatsu Shibasaki
Abstract [Focus Review]
Asian J. Org. Chem. 10.1002/ajoc.201800013

Albert J. Kooistra, Márton Vass, Ross McGuire, Rob Leurs, Iwan J. P. de Esch, Gert Vriend, Stefan Verhoeven, Chris de Graaf
3D-e-Chem: Structural Cheminformatics Workflows for Computer-Aided Drug Discovery [Full Paper]
ChemMedChem 2018, vol. 13, p. 614

Zhoufeng Bian, Sonali Das, Ming Hui Wai, Plaifa Hongmanorom, Sibudjing Kawi
A Review on Bimetallic Nickel-Based Catalysts for CO2 Reforming of Methane [Review]
ChemPhysChem 2017, vol. 18, p. 3117

Turkan Gamze Ulusoy Ghobadi, Amir Ghobadi, Ekmel Ozbay, Ferdi Karadas
Strategies for Plasmonic Hot-Electron-Driven Photoelectrochemical Water Splitting [Review]
ChemPhotoChem 2018, vol. 2, p. 161

An-Na Cho, Nam-Gyu Park
Impact of Interfacial Layers in Perovskite Solar Cells [Review]
ChemSusChem 2017, vol. 10, p. 3687

Jeffrey A. Rood, Sondra E. Hinman, Bruce C. Noll, Kenneth W. Henderson
The Use of Halide-Substituted Anilines for the Formation of Magnesium Imides [Full Paper]
Eur. J. Inorg. Chem. 2008, p. 3935

D. B. Ramachary [Author Profile]
Eur. J. Org. Chem. 10.1002/ejoc.201800182

46. Deutscher Lebensmittelchemikertag 2017 in Würzburg [Tagung]
Lebensmittelchemie 2018, vol. 72, p. 1

Peter Chen
Chemistry 4.0 [Leitartikel]
Nachr. Chem. 2018, vol. 66, p. 203

Ira Caspari, Gisela Weber-Peukert, Nicole Graulich
Der Einsatz von Modellen zum Erkenntnisgewinn / Eine Unterrichtseinheit zur Förderung der Modellkompetenz im Kontext „Batterie“ unter explizitem Einbezug von Schülervorstellungen [Aus der Schule]
CHEMKON 2018, vol. 25, p. 23

Catharina Goedecke
Why Does Iodine Turn Starch Blue?
ChemViews Magazine 2016

Most cited articles from each ChemPubSoc Europe, ACES, and GDCh journal


2016

 


Shoujun Zhu, Qingnan Meng, Lei Wang, Junhu Zhang, Yubin Song, Han Jin, Kai Zhang, Hongchen Sun, Haiyu Wang, Bai Yang
Highly Photoluminescent Carbon Dots for Multicolor Patterning, Sensors, and Bioimaging
Angew. Chem. Int. Ed. 2013, vol. 52, pp. 3953–3957

Balayeshwanth R. Vummidi, Jawad Alzeer, Nathan W. Luedtke
Fluorescent Probes for G-Quadruplex Structures [Review]
ChemBioChem 2013, vol. 14, pp. 540–558

Zhi-Yuan Gu, Jihye Park, Aaron Raiff, Zhangwen Wei, Hong-Cai Zhou
Metal–Organic Frameworks as Biomimetic Catalysts [Minireview]
ChemCatChem 2014, vol. 6, pp. 67–75

Anthony J. Arduengo, Roland Krafczyk
Auf der Suche nach Stabilen Carbenen [Organische Chemie]
Chem. Unserer Zeit 1998, vol. 32, pp. 6–14

Marc Steinmetz, Stefan Grimme
Benchmark Study of the Performance of Density Functional Theory for Bond Activations with (Ni,Pd)-Based Transition-Metal Catalysts [Full Paper]
ChemistryOpen 2013, vol. 2, pp. 115–124

Philipp Scharf, Jens Müller
Nucleic Acids With Metal-Mediated Base Pairs and Their Applications [Review]
ChemPlusChem 2013, vol. 78, pp. 20–34

Philipp Kaiser, Rajabhau?Bajirao Unde, Christoph Kern, Andreas Jess
Production of Liquid Hydrocarbons with CO2 as Carbon Source based on Reverse Water-Gas Shift and Fischer-Tropsch Synthesis [Research Article]
Chem. Ing. Tech. 2013, vol. 85, pp. 489–499

Xiaosi Zhou, Yu-Guo Guo
Highly Disordered Carbon as a Superior Anode Material for Room-Temperature Sodium-Ion Batteries [Communication]
ChemElectroChem 2014, vol. 1, pp. 83–86

Chuanxi Wang, Zhenzhu Xu, Chi Zhang
Polyethyleneimine-Functionalized Fluorescent Carbon Dots: Water Stability, pH Sensing, and Cellular Imaging [Full Paper]
ChemNanoMat 2015, vol. 1, pp. 122–127

Konggang Qu, Jiasi Wang, Jinsong Ren, Xiaogang Qu
Carbon Dots Prepared by Hydrothermal Treatment of Dopamine as an Effective Fluorescent Sensing Platform for the Label-Free Detection of Iron(III) Ions and Dopamine [Full Paper]
Chem. Eur. J. 2013, vol. 19, pp. 7243–7249

Yinuo Wu, Jun Wang, Fei Mao, Fuk Yee Kwong
Palladium-Catalyzed Cross-Dehydrogenative Functionalization of C(sp2)–H Bonds [Focus Review]
Chem. Asian J. 2014, vol. 9, pp. 26–47

Naohiko Yoshikai, Ye Wei
Synthesis of Pyrroles, Indoles, and Carbazoles through Transition-Metal-Catalyzed C–H Functionalization [Review]
Asian J. Org. Chem. 2013, vol. 2, pp. 466–478

Lluís Ballell, Robert H. Bates, Rob J. Young, Daniel Alvarez-Gomez, Emilio Alvarez-Ruiz, Vanessa Barroso, Delia Blanco, Benigno Crespo, Jaime Escribano, Rubén González, Sonia Lozano, Sophie Huss, Angel Santos-Villarejo, José Julio Martín-Plaza, Alfonso Mendoza, María José Rebollo-Lopez, Modesto Remuiñan-Blanco, José Luis Lavandera, Esther Pérez-Herran, Francisco Javier Gamo-Benito, José Francisco García-Bustos, David Barros, Julia P. Castro, Nicholas Cammack
Fueling Open-Source Drug Discovery: 177 Small-Molecule Leads against Tuberculosis [Full Paper]
ChemMedChem 2013, vol. 8, pp. 313–321

Peter Politzer, Jane S. Murray
Halogen Bonding: An Interim Discussion [Review]
ChemPhysChem 2013, vol. 14, pp. 278–294

Volker Hessel, Dana Kralisch, Norbert Kockmann, Timothy Noël, Qi Wang
Novel Process Windows for Enabling, Accelerating, and Uplifting Flow Chemistry [Review]
ChemSusChem 2013, vol. 6, pp. 746–789

Helena J. Shepherd, Gábor Molnár, William Nicolazzi, Lionel Salmon, Azzedine Bousseksou
Spin Crossover at the Nanometre Scale [Microreview]
Eur. J. Inorg. Chem. 2013, pp. 653–661

Junichiro Yamaguchi, Kei Muto, Kenichiro Itami
Recent Progress in Nickel-Catalyzed Biaryl Coupling [Microreview]
Eur. J. Org. Chem. 2013, pp. 19–30

David Schweinfurth, Naina Deibel, Fritz Weisser, Biprajit Sarkar
Mit Klick zu neuen Liganden [Magazin]
Nachr. Chem. 2011, vol. 59, pp. 937–941
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